Beruflich Dokumente
Kultur Dokumente
with Matter
Vasily Arzhanov
Reactor Physics, KTH
Overview
235U
n 2 MeV
n
H2O
235U
E ~ 0.1 eV
400 KeV
Fission
238U 239Pu
Capture
HT 2008 Neutron Interactions Breeding 3
Fission Cross Section
10 4
235
3
U
10
10 2
(barns)
fission
10 1
10 0
capture
10 -1
10 -2 -3
10 10 -2 10 -1 10 0 10 1 10 2 10 3 10 4 10 5 10 6 10 7
Energy (eV)
HT 2008 Neutron Interactions 4
Physical Principles of
Nuclear Reactor
E Leakage
N2
2 MeV
N1
N2 Fast fission
Slowing down
k
n/fission
Energy
N1 Resonance abs.
2.5
Non-fissile abs. Non-fuel abs.
1 eV
Fission
200 MeV/fission
Leakage
HT 2008 Neutron Interactions 5
Important
2.5 n/fiss
f 200 MeV/fiss
MeV = 1.602 10-13 J
Scattering Absorption
63
29 Cu+ 01 n 62
29 Cu+2 1
0n
63
29 Cu(n,2n) 62
29Cu
203
81 Tl+ 01 n 81
200
Tl+4 01 n
203 200
81 Tl(n,4n) 81 Tl
p 14
7 N + 10 n 146C + 11 H 14C production in the atmosphere
d 31
15 P + 10 n 14
31
Si + 21 H
( B)
*
10
5
B+ n 1
0
11
5
73 Li + 42 He
or 10
5
B(n, ) 7 Li
Monoenergetic
beam of neutrons
#
[I ] = 2 Detector
cm s
Vol = AL
L Experiments:
Rcoll(Vol) = INVol
[ ] = cm 2
HT 2008 Neutron Interactions 11
Macroscopic Cross Section
Collimated monoenergetic
neutron beam, n/(cm2sec) I0
x x+dx
t
(total cross-section)
t
Number density of
the target material
HT 2008 Neutron Interactions 14
Solution 1
Rcoll (Vol) = I N Vol
NA 1.6 6.02 10 23
N= = 8 10 22
M 12
#
Rcoll ( Vol) = 2.6 10 24 5 10 5 8 10 22 0.1 0.05 = 5.2 10 5
s
Rcoll 5.2 10 5
Pr {neutroninteracts} = = = 1.04 10 2
I A 5 10 8 0.1
dI ( x) I ( x) I ( x)
= t I ( x) = I ( 0 ) e t x
Pr {Nocollision} = = e t x
dx I (0)
dI ( x)
= Probability of the first collision within dx = t dx
I ( x)
Probability of uncollided 1
flight within distance x
F(x)
P(x) = et x
Probability of at least one
collision within distance x
t x P(x)
F(x) = 1 P(x) = 1 e
0 x
Let p(x)dx be the probability that a neutron will have its first collision in dx around x.
p ( x ) dx = Pr {( Survivesx ) ( Collidesindx )} =
= Pr {Survivesx} Pr {Collidesindx} = e t x t dx
First collision probability: p ( x ) = t e t x p ( x ) dx = 1
0
1
mfp = = xp ( x ) dx = t xe t x dx =
0 0
t
For example, mean free path of 100-keV neutrons in liquid sodium is 11.6 cm.
Collision probability 1
per unit time is
vt = t Mean time
vt
t 1
Alternatively = = t
v vt
HT 2008 Neutron Interactions 20
Cross-Sections of Mixtures
Homogeneous mixture of 2 nuclide species, X and Y.
Probability per unit path length that a neutron collides with X is X = XNX
Probability per unit path length that a neutron collides with Y is Y = YNY
Total probability per unit path length that a neutron collides with either nuclides
= X N X + Y NY It generalizes to = i N i
i
X N X + Y NY
= = = m X + n Y (except elastic scattering)
N N
0.0253 eV 1 MeV
H 21 3
O 4 8
2s(H) + s(O) 46 14
s(H2O) 103 14
s [barn]
Chemical binding is
100
50
2 s (H) + s (O)
0.01 0.1 1 10 E [eV]
I = vn Rcoll ( Vol )
Collision rate: Rt = t I = t vn
Vol
Except for crystals, the interaction of neutrons with nuclei is independent of the angle.
ID
Rt = t ( I A + I B + IC + I D ) = t v ( nA + nB + nC + nD )
n = nA + nB + nC + nD Rt = t vn
IA IC
vn Rx = x
IB n cm 2 s
HT 2008 Neutron Interactions 25
Meaning of cm2 in Flux
I I = vn
#
vn 2
cm s
Rx (r , t) = xvn(r , t) = x(r , t)
# #
n(r , t) 3 (r , t) v n(r , t) 2
cm s cm
# #
n(r , E, t) 3 (r , E, t) v n(r , E, t)
cm J s cm2
J
# #
n(r , E, , t) 3 (r , E, , t) v n(r , E, , t)
cm J sr s cm2
J sr
P(t) = f f (r , E)vn(r , E, t)dEd3r
V 0
J 1 # J
P = 2
Jcm = = W
3
# cm scm J s
P = f R f V = f f V
MeV J 1 #
( )
3
P = 200 1.6 10 13 0.1 1013 2
80cm = 16.4 MW
# MeV cm cm s
Scattering s Absorption a
t = s +a
Fe +
26 26 56 26
26 (radiative capture) 24
22
Fe + 2n
Energy, MeV
56
26
(n,2n) reaction 20
18
16
14
12
10
8
Cross-sections of nuclear reactions exhibit maxima at certain 6
incident neutron energies. The maxima are called resonances. 4
2
0
Regions:
Potential scattering e = 4 R2
Elastic scattering cross-section
as a function of Resonances
incident neutron energy, E
Smooth region
Resonance
region
e = 4 R2
Potential scattering
~50 keV
0.01 eV 100 keV Smooth
region
HT 2008 Neutron Interactions 38
Elastic Scattering for 238U
Density increases
~10 eV
1 eV 1 keV
100
10
1
Neutron Interactions
0,1
10 20 30 40 50
Incident Energy (eV)
Incident neutron data / ENDF/B-VII.0 / U235 / Resonances /
Resonances data Resolved parameters : 1.0E-5 < E < 2250.0
1000 T=300.0 K
500
235U
100
Resonances (b)
50
10
5
1
0,5
0,1
10 20 30 40 50
Incident Energy (eV)
E
0
(eV)
50
HT 2008
Summary for
Resonance Levels
For light nuclei resonance levels are scarce with
distance of about 100 keV or more. For heavy nuclei
distance between the levels is of the order of few eV
Density of levels increase with energy. Pronounced
effect of EVEN - UNEVEN nuclei. When neutrons
interact with nuclei with EVEN mass number
resonances are at larger distances than for UNEVEN
mass numbers
1 MeV
50 KeV
Ground
Li, Be 238U
Smooth region
There are a few important nuclei that do not show exact 1/v behaviour.
They are called non-1/v absorbers.
1/v region
r2 g n
( E) =
4 ( E Er )2 + 2 4
Total width, = n +
x,max Er
x ( E) =
max E Er
2
E
+1
2
max
2 s,max
s ( E) = 2
E Er
+1
2
Er E
HT 2008 Neutron Interactions 48
Charged-Particles Reactions
En > 9 MeV
As a rule, the (n,p), (n,) are endothermic and do
not occur below some threshhold energy. Their 16
8 O ( n, p ) N
16
7
7 sec
8O +
16
cross-sections tend to be small, even above the
threshhold, especialy for heavier nuclei.
E > 67 MeV
6
3 Li ( n, ) 31 H 1/v absorber
Tritium production
Several orders
E
239Pu
Total
Fission
Capture
Elastic
Inelastic
s is constant up to 10 keV.
is 1/v up to 1 MeV.
1/v region
0.253
( 1eV ) = 0.332 = 0.0528 b
1
Total collision rate Rt = t ( E ) v( E)n( E)dE
0
Absorption collision rate Ra = a ( E ) v( E)n( E)dE
0
Ra = a ( E ) v( E)n( E)dE = a ( E0 ) v0 n( E)dE = a ( E0 ) v0 n
0 0
For 1/v absorbers, the absorption rate is independent of the energy distribution.
Equivalently, the absorption rate is the same as that for a monoenergetic beam of
neutrons with arbitrary energy E0 and intensity v0n.
Ra = a ( E0 ) 0
0 v0 n
HT 2008 Neutron Interactions 56
Non-1/v Absorbers
There are a comparatively few important non-1/v absorbers.
Ra = a ( E ) v( E)n( E)dE It is dependent on the neutron energy distribution n(E).
0
Ra = ga (T ) a ( E0 ) 0
T C ga ga ga ga ga gf ga gf ga ga gf
20 1.3203 1.0192 1.1581 1.6170 0.9983 1.0003 0.9780 0.9759 1.0017 1.0723 1.0487
100 1.5990 1.0350 1.2103 1.8874 0.9972 1.0011 0.9610 0.9581 1.0031 1.1611 1.1150
200 1.9631 1.0558 1.2360 2.0903 0.9973 1.0025 0.9457 0.9411 1.0049 1.3388 1.2528
400 2.5589 1.1011 1.1864 2.1854 1.0010 1.0068 0.9294 0.9208 1.0085 1.8905 1.6904
600 2.9031 1.1522 1.0914 2.0852 1.0072 1.0128 0.9229 0.9108 1.0122 2.5321 2.2037
800 3.0455 1.2123 0.9887 1.9246 1.0146 1.0201 0.9182 0.9036 1.0159 3.1006 2.6595
1000 3.0599 1.2915 0.8858 1.7568 1.0226 1.0284 0.9118 0.8956 1.0198 3.5353 3.0079
Ra = ga (T ) a ( E0 ) 0
A small indium foil is placed in a reactor where 2200 m/s flux is 51012 n/cm2s. The neutron
density can be represented by a Maxwellian distribution with a temperature of 600 C. At
what rate are neutrons absorbed per cm3 in the foil? NIn = 0.03831024 and a(E0) = 194 b.
97%
Channel 1: 252
98 Cf (6 MeV)
Channel 2: 3% 252
98 Cf 3.8 n (185 MeV)
FP
FP
HT 2008 Neutron Interactions 63
Fission and Spallation
Elastic
scattering
m ( v0 + v1 ) = MV1
Applying collision laws 2m
Chadwick derived: 1 1
V1 = v0
2 MV1 = 2 m ( v0 + v1 ) M+m
2 2 2
2
1 H+ 11 H+ 01 n Q = 2.226 MeV
9
4 Be + 84 Be + 01 n Q = 1.666 MeV