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Abstract
Multicondition-driven mechanisms may produce pyroclastic deposits varying in fundamental properties such as
dispersal, grain size, vesicularity and morphology of juvenile clasts, and the abundance of lithic or wall rock ejecta
(xenoliths). Volcanic ash particles from different fragmentation mechanisms have different surface textures and
morphologies. The analysis of the volcanic clast shape remained largely qualitative. A new method for ash particle
characterization based on quadtree decomposition and surface gradient analysis is introduced. The approach is applied for
assessing fragmentation mechanisms operating during eruptions. The surface descriptor variables like the number of
quadtree blocks (nQT), the mean block size (mQT), the standard deviation of block sizes (sQT) and the surface descriptors
derived from gradient analysis seem to be suitable for quantifying the structural changes of the ash surface due to variable
explosion conditions. These parameters are presented in volcanology as distinctive key parameters for different eruption
types. This may enrich our capabilities for effective prediction for the basis of planning to overcome the impending danger
of eruptions.
r 2005 Elsevier Ltd. All rights reserved.
0098-3004/$ - see front matter r 2005 Elsevier Ltd. All rights reserved.
doi:10.1016/j.cageo.2005.10.013
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mass ratio of interacting water and magma, sub- the presence of such glass shapes show that
plinian dispersal of pumice and air falls, base surge phreatomagmatic ash is formed by thermal con-
deposits with dune and anti-dune structures, cross- traction and shattering of glass which inhibits
beddings, bread-crust bombs are observed. vesiculation. The very drastic increase in viscosity
and the increase in solubility due to the decrease
1.2. Volcanic ash formation in temperature prevent volatiles from exsolution
(Fisher and Schminke, 1984). The widely varying
Volcanic ashes are the particles with average clast vesicularities reect complex variations in the
diameters o2 mm those produced during volcanic relative timing of vesiculation and water-induced
eruptions by mechanical fragmentation of magma fragmentation. Magmawater interaction at an
and/or country rock. There are three main mechan- early stage greatly reduces the vesicularity indices
isms of volcanic ash formation: (1) the release of (o40%) and broadens the ranges (as high as 80%),
gases due to decompression within the magma whereas late-stage interaction has only a minor
ascending to the surface (magmatic eruptions), effect on the index and broadens the range to a
(2) chilling and explosive fragmentation of magma limited extent (Houghton and Wilson, 1989).
during contact with ground and surface water or Deposits from phreatomagmatic eruptions are
ice and snow (phreatomagmatic eruptions), and characteristically ne-grained, although coarse-
(3) the comminution and ejection of particles from grained lapilli- and tuff-breccias are common in
vent walls or crater debris during eruptions of steam some deposits (Fisher and Schminke, 1984). Walker
and hot water (phreatic eruptions). Volcanic ash can (1973) shows that the median diameters is less than
be produced by one or more of these mechanisms 1 mm in about 75% of the samples from phreato-
(Heiken and Wohletz, 1985). magmatic explosions in Azores and Iceland. In any
The term phreatomagmatic was introduced by fragmentation mechanism the generated particles
Stearns and MacDonald (1946) in reference to sizes reect the kinetic energy available (i.e., the
explosions resulting from the conversion of ground- fragmentation energy density). Consequently, ne
water to steam by ascending magma. A phreato- ash provides information on fragmentation me-
magmatic explosion refers to natural phenomena chanisms that are the most energetic and related to
produced by the interaction of magma or magmatic the highest explosive energy release (Zimanowski
heat with an external source of water, such as et al., 2002). With increasing water interaction,
surface body or an aquifer (MacDonald, 1972; phreatomagmatism increases in explosivity. The
Sheridan and Wohletz, 1981). The products are abundance of ne ash (o63 mm) increases from 5
water, steam, juvenile clasts and brecciated country- to over 30% as water interaction reaches an
rocks (accessory and/or accidental xenoliths). explosive maximum (Wohletz, 1983).
Accessory particles are fragmented co-magmatic An important consideration is that both magmatic
volcanic rocks from previous eruptions of the same and phreatomagmatic fragmentation mechanisms
volcano. Accidental fragments are derived from the may operate during an eruption. This situation was
subvolcanic basement and therefore may be of any illustrated by Self and Sparks (1978) for phreatopli-
composition (Fisher and Schminke, 1984). Phreato- nian silicic eruptions in which magma is initially
magmatic deposits are rich in xenoliths indicating disrupted by exsolution and expansion of magmatic
the fragmentation of country rock with high volatiles, producing relatively coarse-grained pyro-
energies due to abundant water (vapour). clasts. Further fragmentation (ne-grained pyro-
Volcanic ash deposits produced during these clasts) is caused by explosive interaction with
eruptions are unique and their characteristics may water. Theoretical consideration of experimental
be used to interpret eruptive mechanisms. The fragmentation mechanisms suggests that stress waves
phreatomagmatic deposits contain grains that have produced by high-pressure, vaporization of water at
been signicantly affected by a variety of processes the magma/water interface may, in part, induce
related to their formation, transport and alteration. vesiculation in the melt (Heiken and Wohletz, 1985).
The common shapes of glass pyroclasts can be
ascribed to varying energies and modes of contact of 1.3. Classification of volcanic ash
water with magma, including blocky-equant, moss-
like, plate-like and drop or spherical (Wohletz, Scanning electron microscopy (SEM) provides a
1983). Considering the explosive mechanisms and method for classifying volcanic ash based upon
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surface morphology and texture (Wohletz and paper, the quadtree representation of data is
Krinsley, 1982). Heiken (1972, 1974), Wohletz concerned with the representation of region data.
(1983) and Heiken and Wohletz (1985) presented A region quadtree is a representation of a regular
the most extensive SEM studies of pyroclast shapes partitioning of space where regions are split
and found a marked difference in grain morphology recursively until there is a constant amount of
between magmatic and phreatomagmatic ashes. information contained in them (Wang and Arm-
While some forms of glassy particles refer to strong, 2003). Each quadtree block (also referred as
phreatomagmatic or magmatic fragmentation, the a cell, or node) covers a portion of space that forms
lack of clear key structures prevents the classi- a hypercube in d-dimensions, usually with a side
cation (Dellino and La Volpe, 1996). The success in length that is a power of 2. Quadtree blocks may be
the discrimination depends on the experience of further divided into 2d sub-blocks of equal size; i.e.,
microscopist (Sheridan and Marshall, 1983). Thus the sub-blocks of a block are obtained by halving
the analysis of the volcanic clast shape remained the block along each coordinate axis, forming an
largely qualitative (Marshall, 1987). adaptive grid (Fig. 1A). A quadtree may be
Dellino and La Volpe (1996) introduced new considered as an extended 2d-ary tree, i.e., a tree
methods using particle outline parameters such as in which every non-leaf node has 2d children
elongation, roundness, compactness and rectangu- (Fig. 1B). A quadtree is thus a tree, where the
larity to dene the particle forms from Monte branch structure is based on space coverage
Pilato-Rocche Rosse. The outline parameters are (Hjaltason and Samet, 1999).
inuenced by transportation mechanisms (Dellino Gradient analysis is also suitable for describing
and La Volpe, 1996) and the effects of transporta- texture orientation. Similar methods have been used
tion abrasion may be misinterpreted as fragmenta- to detect the orientation of short-bre composites
tion features or vice versa. (Gadala-Maria and Parsi, 1993) and actin bres in
cytoskeletal structures (Yoshigi et al., 2003). This
1.4. Texture characterization may be valuable information for differentiating
between textures having the same greylevel varia-
Several texture descriptors have been developed tion. The gradient analysis is based on Sobel
to characterize the detailed surface structure of, e.g. operators as described by Gonzalez and Woods
aluminium (Lee et al., 1998), aggregate (Rao et al., (1993) and implemented by Chinga et al. (2003).
2003), wear particles (Stachowiak, 1998) and paper This study introduces a new method for ash
surfaces (Chinga et al., 2003; Chinga, 2004). Fractal particle characterization based on a quadtree
dimension, autocorrelation, gradient analysis, band- decomposition approach and gradient analysis.
pass ltering, wavelet analysis, roughness statistics The approach is applied for assessing fragmentation
and quadtree decomposition have been applied to mechanisms operating during eruptions. The calcu-
assess complex surface structures (Panozzo Heil- lated quadtree variables like the number of blocks
bronner, 1992; Costa, 2000; Chinga et al., 2003;
Chinga, 2005). In this respect, quadtree decomposi-
tion seems to be an easy, intuitive and powerful
technique for characterizing the horizontal and
vertical variation of surfaces (Chinga, 2005).
Hierarchical data structures are becoming in-
creasingly important representation techniques in
the domains of computer graphics, image proces-
sing, computational geometry, geographic informa-
tion systems, and robotics. They are based on the
principle of recursive decomposition. One such data
structure is the quadtree (Samet, 1984). In the elds
of image processing, computer graphics, and remote
sensing two-dimensional point and region data are
Fig. 1. (A) Block decomposition; (B) tree structure of a simple
often indexed using quadtrees (Samet, 1990). quadtree, where leaf blocks are labeled with numbers and non-
Currently, quadtrees are used for point data, leaf blocks with letters (reproduced from Hjaltason and Samet,
regions, curves, surfaces, and volumes. In this 1999).
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(nQT), the mean block size (mQT) and the standard clast density is that of the most vesiculated
deviation of block sizes (sQT), as well as surface fragments. The density of juvenile fragments was
descriptors derived from gradient analysis seem to measured with a pycnometer after coating frag-
be suitable for quantifying the structural changes of ments with a silicon-based aerosol which has
the ash surface due to variable explosion conditions. negligible mass. About 10 measurements per sample
These parameters are presented in volcanology as were carried out in the 4-8 mm grain classes. The
distinctive key parameters for different eruption mean values were then considered. The vesicularity
types. index (V%) was calculated using the method of
Houghton and Wilson (1989). The results for three
2. Materials and methods samples N1, N2 and N3 are given in Fig. 2. The
percentages of material ner than 1 mm in samples
2.1. Sample description show the decreasing grain size through the explo-
sion produced the last sample (N1) with abundant
Three samples denoted Nemrut1 (N1), Nemrut2 water interacted with magma. The decreasing
(N2) and Nemrut3 (N3) and indicating the changes median diameters also point the increasing water
in eruption styles were selected. Samples were taken interaction through the eruption. The increasing
from the very proximal location, the interior side of xenolith contents through the last sample (N1) also
the caldera rim. Unvesiculated and rounded parti- exhibits increasing fragmentation of country rocks
cles with hydration cracks are common in sample with increasing energies due to the abundant water
Nemrut1 which was collected from a base surge (vapour). The increasing densities and decreasing
deposit. Few vesicles on Nemrut1 are lled with vesicularities of particles demonstrate the increasing
adhering dust. Particle morphologies of this sample role of external water versus magmatic volatiles in
exhibit the water effect. Sample Nemrut2 is highly driving explosive eruption.
vesiculated. The tubular vesicles are prevalent
indicating the effects of a magmatic origin. Nemrut3 2.2. Sample preparation and image acquisition
is also highly vesiculated, and exhibits tubular
vesicles. It is not easy to separate the phreatoplinian The samples from the three eruption types were
samples Nemrut2 and Nemrut3 with naked eye. In washed to remove any organic, loosely adhered and
the eld, the arrangement of deposits from base to cementing material. Depending upon the freshness
top is Nemrut3, Nemrut2 and Nemrut1 indicating of the grains, washing included soaking in hot,
the progressive increase in amount of water inter- dilute HCl and acetone or cleaning in acetone using
acting with magma. ultrasound for not more than 4 min to preserve
In addition, 160 samples were collected from the grain edges (Heiken and Wohletz, 1985). The
Nemrut Volcano (Turkey) for ash details determi- samples were mounted on stainless-steel stubs using
nation. The samples from Nemrut show differences double stick tape and coated with carbon in order to
in bed structures, grain sizes, xenolith contents, counteract grain surface charging while scanning
density and vesiculation indicating the continuous with the electron beam.
changes in the eruption style (for details see Ersoy et A CAMECA SU-30 operating at secondary
al., in preparation). The grain size analysis includes electron mode with 17 KeV was used at Hacettepe
drying, sieving and weighting of the different grain- University (Turkey) to take the whole grain and
size classes in phi scale. Percentage of tephra ner detailed surface photographs. The grain size interval
than 1 mm and median diameter (Md) were used to of 250355 mm was selected for comparing the
show the ner grain sizes related to high explosion textures with other studies (Wohletz, 1983; Heiken
energies due to abundant water. Particles of the 2 4 and Wohletz, 1985). Ten scanning electron images
and 4 8 mm size classes were hand-picked under a were acquired from each sample.
binocular stereoscope for particle analysis. The
different components were weighed and the weight 2.3. Image processing and analysis
percentage was calculated. The components are
juvenile vesicular grains, unvesicular juvenile clasts Image processing and analysis of the secondary
and brecciated country-rocks (xenoliths). The dense electron images (SEI) were performed using the
rock equivalent (DRE) density has been determined ImageJ program (Rasband, 2004). The SurfCharJ
on non-vesicular, dense grains, while the average plugin (Chinga et al., 2003) was used for surface
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940 O. Ersoy et al. / Computers & Geosciences 32 (2006) 936946
Fig. 2. Determination of volcanic ash details. (A) Percentage of tephra ner than 1 mm; (B) xenolith ratio; (C) density; (D) vesicularity
index.
assessment and gradient analysis. The SurfCharJ image is based on obtaining the partial derivatives
plugin describes surface representations by calculat- at every pixel. Derivatives may be implemented in
ing surface statistics like the standard deviation, the several ways, however, the Sobel operators have the
skewness, the kurtosis, mean greylevel (mGL) and advantage of providing both differencing and a
standard deviation of greylevel values (sGL). The smoothing effect (Gonzalez and Woods, 1993). This
statistics were calculated for all the images. The smoothing effect of Sobel operators is particularly
standard deviation is given by attractive due to the noise enhancing effect of
!1=2 derivatives. Derivatives based on Sobel operator
1 Xw X h
2 masks are
Standard deviation z zxy ,
wh x1 y1
G x z7 2z8 z9 z1 2z2 z3 (2)
(1) and
where w and h are the image dimensions, z the
G y z3 2z6 z9 z1 2z4 z7 , (3)
mean greylevel and zxy local greylevel at local
position x,y. For details about the surface descrip- where the zs represent the greylevels overlapped by
tors yielded by the SurfCharJ plugin see Chinga the 3 3 mask at any location in an image. The
et al. (2003). numbering of the z-values corresponds to the
A gradient analysis based on Sobel operators was sequence from left to right, top to bottom in a
performed. The computation of the gradient of an 3 3 mask. The direction at the location of the
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O. Ersoy et al. / Computers & Geosciences 32 (2006) 936946 941
Fig. 3. Structure orientation analysis. (A) Original greylevel image; (B) azimuthal image; (C) polar plot based on frequency of gradients.
Bar in A 100 mm.
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942 O. Ersoy et al. / Computers & Geosciences 32 (2006) 936946
the variances within the groups (replicates). The different structures may have the same greylevel
ANOVA tests for the accepted variables are given in variation, but different texture. This is exemplied
Figs. 46. The greylevel standard deviation (sGL), in Fig. 7. A gradient analysis revealed signicant
the form factor (FF) and the number of quadtree differences between the structures (Fig. 8). Fig. 7A
blocks (nQT) seem suitable for differentiating has a texture with clear orientation compared to
between samples, having p-values well below 0.05 Fig 7B.
with a 95% condence interval (CI). Though both images have the same global sGL,
Among all the evaluated surface texture descrip- there are also clear differences with respect to the
tors, the greylevel standard deviation seems to give local greylevel standard deviation. This is exempli-
the best differentiation between the samples. How- ed in Fig. 9 where Fig. 9B has larger areas with
ever, this parameter alone is insufcient to describe lower greylevel variation, thus having larger and
the structure in detail. The greylevel and greylevel fewer blocks after the corresponding quadtree
variation may vary signicantly depending on the decomposition.
settings used for image acquisition. Besides, two All the presented texture descriptors (sGL, nQT
and FF) seem to model the transition from a drier
explosion to a wetter explosion. In addition, a data
reduction method, R-mode factor analysis was
performed on the three variables. The term factor
analysis was rst introduced by Thurstone, 1931.
Fig. 5. ANOVA of form factor (FF) variable. Samples Nemrut1 Fig. 7. Two images having same greylevel standard deviation,
(N1), Nemrut2 (N2) and Nemrut3 (N3) are included in analysis. i.e., 36. (A) Image from N2 sample showing a clear texture
Mean values are given with corresponding 95% CI. orientation; (B) image from N3 sample. Bar 100 mm.
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O. Ersoy et al. / Computers & Geosciences 32 (2006) 936946 943
Fig. 10. Discriminating diagram based on texture classication. Diagram shows a clear transition between wetter and drier stages.
Samples from Nemrut1 (N1), Nemrut2 (N2) and Nemrut3 (N3) are included in diagram.
Fig. 11. Discriminating diagram based on particle outlines. No differentiation between three given stages is observed. Samples from
Nemrut1 (N1), Nemrut2 (N2) and Nemrut3 (N3) are included in diagram.
statistical analysis, articial intelligence and study to the varying energies, modes of contact of water
on high dimensional data. and chemistry of magma. Multicondition-driven
Simple and well-dened surface descriptors have mechanisms may produce pyroclastic deposits
been presented in this study. Parameters derived varying in fundamental properties such as dispersal,
from a quadtree decomposition approach seem to grain size, vesicularity and morphology of juvenile
be suitable for describing ash texture. Complemen- clasts, and the abundance of lithic or wall rock
tary information is obtained by performing a ejecta (xenoliths).
gradient analysis. The proposed image processing The products under the inuence of modifying
and analysis is simple to implement and requires conditions can be discriminated from each other by
little subjective intervention. using the properties mentioned above. Among the
Although, the common shapes of glass pyroclasts criteria used to distinguish the products of dry
in phreatomagmatic explosions such as blocky- magmatic eruptions from wet phreatomagmatic
equant, moss-like, plate-like and drop or spherical eruptions, the vesicularity of the juvenile clasts is
may be used as key structures, they are uncom- generally considered to be high in the former and
mon, indenable or absent in some products related lower in the latter case (Walker and Croasdale,
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O. Ersoy et al. / Computers & Geosciences 32 (2006) 936946 945
1972; Houghton and Wilson, 1989). Even though it Cattell, R.B., 1966. The scree test for the number of factors.
is necessary to take all fundamental properties into Multivariate Behavioral Research 1, 245276.
consideration in such variable mechanisms, the Chinga, G., 2004. Detailed characterisation of paper surface
structure for gloss assessment. Journal Pulp Paper Science 30
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descriptors derived from gradient analysis, which Chinga, G., 2005. A quadtree decomposition approach for
may be directly related to vesicularity, clustered the surface assessment. Pattern Analysis and Applications, in
ash particles between two end member mechanisms. press.
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reconstructing fragmentation and transportation mechanisms
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Acknowledgements ment, TR-4033, University of Maryland, College Park, MD.
Available from http://www.cs.umd.edu/hjs/pubs/bulkload.
This work beneted from a research grant of pdf.
Hacettepe University Research Foundation (Project Houghton, B.F., Wilson, C.J.N., 1989. A vesicularity index for
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