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Our goal is to analyze nuclear reactors. In addition to the description of the physical processes,
we need to come up with a mathematical form (i.e., a set of equations) that will help us to quan-
tify what is happening in the reactor core. The equations we use will contain mathematical
descriptions of the rates at which neutrons interact with the nuclei. Thus, we must describe such
interactions mathematically.
We will begin with “microscopic” cross sections, which describe the likelihood that a neutron
will interact with a given nucleus. Therefore, “microscopic” cross sections will depend on the
properties of target nuclei and neutrons. For our purposes, the target nucleus is assumed to be at
rest in the laboratory system. If the thermal motion of the target nucleus cannot be neglected, we
introduce the “relative” neutron velocity with respect to target nucleus. The cross sections depend
only on this relative neutron velocity. Consider a beam of neutrons, all with the same velocity,
normally (perpendicularly) incident on a very thin plate of some material:
N
FIGURE II.16. A monoenergetic parallel neutron beam incident normally on a thin target
II.28
We shall assume that the target is so thin that all nuclei are “visible” to the incident neutrons ––
no nucleus is hidden behind another nucleus. We define:
The rate at which neutrons collide with nuclei must be proportional to I (the rate at which neu-
trons strike) and to NΔx (the areal density of target nuclei), i.e.:
2
colliding neutrons cm neutrons nuclei
- = ------------------
------------------------------------------ -------------------
- -------------
- [ cm ] (II. 32)
cm s
2 nucleus cm s
2
cm
3
where the symbol σ to represent the constant of proportionality. We have determined that σ must
have units of area per nucleus. We refer to σ as a “microscopic cross section”. We tabulate micro-
scopic cross sections in units of barns, with 1 barn defined to be 10–24 cm2.
If neutrons were classical point particles and nuclei were classical spheres, σ would simply be the
cross-sectional area of each nucleus. (Since a nuclear radius is on the order of 10–12 cm, one barn
is on the order of the cross-sectional area of a nucleus.) In reality, neutron-nuclear collisions are
described by quantum-mechanical laws, and they have little to do, in general, with the geometry
of a nucleus. However, it is still useful to think of σ as the effective area that a nucleus presents to
a neutron.
the relative speed between the neutron and the nucleus, and
the target nuclide.
In the preceding discussion we were looking at the total rate at which neutrons interact with
nuclei, without distinguishing between different kinds of interactions (elastic scattering, fission,
inelastic scattering, capture, etc.). The σ that we used above is called the microscopic total cross
II.29
section, and is denoted σt. It can be thought of as the sum of microscopic cross sections for vari-
ous specific interactions:
where: σt = total cross section, σa = absorption cross section, σs = scattering cross section, σγ =
radiative capture cross section, σf = fission cross section, σn,2n = (n,2n) cross section, and σn,α =
(n,alpha) cross section.
Σx = N σx [cm–1],
for each different type, x = {t, a, s, γ, f, ...}, of interaction. Note that macroscopic cross sections
have units of inverse length: [nuclei/cm3] • [cm2/nucleus] = cm–1.
In addition to their convenience, macroscopic cross sections have an important physical interpre-
tation. Let us return to our uniform beam of mono-energetic neutrons incident normally upon a
target. This time we allow the target to be thick. We define:
I0 I(x)
x=0 x x+dx
FIGURE II.17. Monoenergetic parallel neutron beam incident normally on a thick target
II.30
We have:
dI
------ = – N σ t I ( x ) = – Σ t I ( x ) (II. 34)
dx
which is of exactly the same form as the equation that governs radioactive decay. Its solution is
easily found by integration:
–Σt x
I ( x) = I 0e (II. 35)
where I0 is the uncollided intensity at x = 0. Thus, uncollided neutrons are exponentially attenu-
ated as they try to pass through matter. This is analogous to the exponential decay of radioactive
nuclides as they try to pass through time.
It follows from their definition that macroscopic cross sections are additive in the same way that
microscopic cross sections are:
Σ t = Σ a + Σ s = ( Σ γ + Σ f + Σ n, α + … ) + ( Σ el + Σ in ) (II. 36)
In addition, given a mixture of nuclides Y1, Y2, ..., with number densities N1, N2, ..., and micro-
scopic cross sections σx1, σx2, ..., for any type, x, of interaction, the macroscopic cross section for
the mixture can be calculated as:
Finally, we have already noted that microscopic cross sections for a given nuclide will depend on
the relative speed between the neutron and the nucleus. Actually, it is convenient and customary
to tabulate cross sections in terms of the neutron energy E = mv2/2 instead of the speed v. Thus,
we have:
σx = σx(E).
We note further that in general, atomic number densities in practical problems will depend on
space and time. Thus, in general,
Σ x = N ( r, t )σ x ( E ) = Σ x ( r, E, t ) ) (II. 37)
II.31