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To cite this article: Michael Koch & Gernot Krammer (2008) The Permeability Distribution (PD)
Method for Filter Media Characterization, Aerosol Science and Technology, 42:6, 433-444, DOI:
10.1080/02786820802172053
433
434 M. KOCH AND G. KRAMMER
Strangert (1978), Leubner and Riebel (2001), and Hoff et al. an altered flow field with filter cake present is calculated, and
(2005) find that the pressure drop increases rapidly immediately further cake build up can be simulated. Thus, an inhomogeneous
after initiating filtration starts; however, the rate of increase slows filter cake gradually develops around the perforation. The appar-
as the filter cake develops. Leubner and Riebel (2001) ascribe ent permeability of the growing filter cake is calculated and for
their experimental findings to inhomogeneities in the filter cloth, thin cakes the apparent permeability of the inhomogeneous filter
but provide little detail. The time variation of the pressure drop cake is significantly lower than the corresponding permeability
across a filter is decisive for the operating pressure drop level of a homogeneous cake with the same mean thickness. The ap-
of a filter. A pressure drop curve with a decreasing slope, but parent permeability approaches the mean value as cake growth
the same asymptotic slope, is always above the linear curve in- proceeds. This again implies that at a constant flow rate and con-
crease. Thus, a filter actually exhibiting such a curved pressure stant upstream solid concentration, i.e., time-linear mean cake
drop profile will operate during filtration cycles at an average growth, the pressure drop is initially increasing faster, since the
pressure above the ideally expected linear case. pressure drop and the permeability are inversely proportional.
Gradual cake compression cannot account for the observed Here the inhomogeneity of the filter cake is not exclusively at-
pressure drop profiles, since it would increase the pressure drop tributed to the pore structure of the medium, but also to the
slope. Increasing pressure drop slopes are reported to originate upstream flow. The modeling of the filter medium as uniform
from depth filtration too, where particles are deposited inside the sieve with regular holes, i.e., as the combination perforation–
filter cloth. Both processes increase specific dust cake resistance impermeable plate, is not directly applicable fabric filter media,
(Schmidt 1997). and Dufrêche et al. (2002) rightfully mention their main applica-
Chen et al. (2001) present a detailed experimental study of tion in membrane filtration. Although this model is not applied
the pressure drop over three cleanable needlefelt filter media that to the complex structure of a fabric filter medium, its findings
were challenged with monodisperse dust. They report a rather are phenomenologically interesting for fabric filtration as well.
fast initial pressure drop increase, that slows over the course of Modeling the filter plant operation introduces another per-
filtration. This effect was observed on all filter media for particle spective on inhomogeneity of the filter. Duo et al. (1997), Dit-
sizes 5, 10, and 20 µm. The initial slope for 5 µm particles tler and Kasper (1999), Kavouras and Krammer (2003), and Mao
was, however, slightly lower, which indicates depth filtration, et al. (2006), for example, propose their respective models. In
possibly because the smallest particles may be able to penetrate these models, the filter area is divided into different model ar-
deeper into the filter medium than larger particles. The rapid eas, each carrying patches of filter cake. The size of each patch
pressure drop increase at the beginning of filtration is ascribed and cake thickness on the patch is derived from the degree of
to inhomogeneous pore filling the filter medium surface; the regeneration and the operational setup of the filter, i.e., whether
rate of increase slows once a homogeneous cake develops. Chen or not the filter is divided into compartments that are cleaned
et al. (2001) hypothesize that a two-stage cake development separately. Since cake patches of different thicknesses impose
within and on top of the pores occurs for the larger particles that correspondingly different flow resistances, an inhomogeneous
they studied. They observed that the deposited particle mass flow situation arises. Darcy’s law typically captures the fluid
at the end of stage one, i.e., pore filtration, did not depend on flow through the filter medium and filter cake. The build up of
the particle size. Stage two is homogeneous filter cake build up a filter cake is governed by the solid mass reaching the filter,
over the entire area of the filter medium. The flow resistance i.e., all particles that are transported to the filter form the filter
increased linearly with decreasing particle size in contrast to cake. Both, compressible and incompressible cakes are simu-
previous reports of a quadratic dependency on size (Kozeny lated. The models proposed in the literature simulate this situa-
1927, cited in Löffler et al. 1988). The experimental findings tion, accounting for the contributions of various mechanisms of
in Chen et al. (2001) suggest that the initial cake build up is the filter operation such as an incomplete filter regeneration (all
inhomogeneous, which may result from an inhomogeneous pore models), a compartmented filter setup (explicitly by Kavouras
structure, but no quantitative analysis is given. and Krammer 2003), an initial depth filtration stage (Mao et al.
Dufrêche et al. (2002) study fluid flow in Stokes regime 2006), and a two-dimensional flow field (Dittler and Kasper
two-dimensionally through a highly idealized porous layer. The 1999). However, the inhomogeneous distribution of the filter
model geometry considered is a uniform sieve with regular per- cake and, thus, of the filter permeability is exclusively attributed
forations, i.e., a flat plate with regularly arranged holes. Fluid to the history of the filter cake, i.e., previous filtration and re-
can only pass through the actual perforation. The streamlines are generation cycles. None of the filter operation models available
correspondingly deflected upstream of the sieve and are concen- in the literature consider, or even describe, an inhomogeneous
trated through the perforation. Cake build up simulations with filter medium itself.
Lagranian particle tracking, neglecting any slip between the fluid This work comprises the deduction of a one-dimensional fil-
and particles, yields a preferential cake development on or close ter model based on flow governed by Darcy’s law that allows for
to the perforation. The deposited cake is treated as continuous inhomogeneous filter medium permeability. The filter medium
porous solid with fixed, isotropic flow resistance properties. Its permeability is taken as a distribution, rather than geometrically
hydrodynamics can be described by Darcy’s law. Subsequently resolved. This distribution can account for pores in the filter
PD METHOD FOR FILTER MEDIA CHARACTERIZATION 435
proportionality factor is the specific cake resistance αm . and the time derivative of Equation (3) is:
1 1
1
= αm · z(t, A) [2] d k(t,A)
d kc (t,A)
kc (t, A) = [7]
dt dt
When a filter cake is present, the fluid flow is determined by Expressing the solid area load term in Equation (6) by Equa-
the combined flow resistances of filter medium and filter cake. tion (5) and subsequently kc (t, A) by k(t, A) using Equation (7)
The flow resistances of filter medium k0−1 (A) and filter cake gives:
kc−1 (t, A) are in series and thus add linearly:
1
1 1 1 d k(t,A)
= + [3] = αm · csol · v(t, A) [8]
k(t, A) kc (t, A) k0 (A) dt
The fluid flow when cake is present is determined by a linear Here the filtration velocity v(t, A) can be expressed by Equa-
relation similar to Equation (1) but with the combined perme- tion (4), which reads:
ability k instead of just k0 :
1
d k(t,A) αm · csol
p(t) = · k(t, A) · p(t) [9]
v(t, A) = k(t, A) · [4] dt ηg
ηg
In this equation, both the permeability and the pressure drop
The permeability depends on both the location on the filter A are time dependent. However, Equation (9) can be rearranged
and the filtration time t. The latter dependency describes the by separating variables. Thereby evaluating the derivative on the
evolution of the permeability as cake build up proceeds. The left-hand side of Equation (9) gives:
mechanistic cake build up is described by solid continuity. In
cake filters, almost all the dust that is transported to the filter is d (k(t, A)) αm · csol
retained on the filter to form a cake. Here it is assumed that the − = · p(t) · dt [10]
k 3 (t, A) ηg
upstream solid concentration is constant, so the filter cake mass
balance reads:
Equation(10) is a differential equation with separated vari-
dz(t, A) ables k(t, A) and p(t), respectively. Integrating from time zero
= csol · v(t, A) [5] to t on the right-hand side and the corresponding permeabilities
dt
on the left-hand side gives:
Equation (5) gives the direct proportionality between cake build
up and flow velocity. 1 1 αm · csol t
− =2· · p(t) · dt [11]
The filter cake depicted in Figure 1b causes, as stated, addi- k 2 (t, A) k02 (A) ηg 0
tional flow resistance. To overcome that increased resistance and
keep the total volume flow constant (constant flow filtration) the Hereby, the relation k(t = 0, A) = k0 (A) is used, reflecting that
pressure drop increases. In classical filtration theory a homoge- at time t = 0 the permeability relates only to the permeability
neous filter medium and a homogeneous filter cake build up give of the filter medium (cf. Equation [1]). In Equation (11) the
a linear pressure drop increase (Löffler et al. 1988). However, right-hand side is only time dependent, i.e., it does not show any
if the filter medium is inhomogeneous but an internally homo- dependency on the filter area. That implies that the evolution of
geneous cake builds up the pressure drop increases nonlinearly the permeability with the distributed initial value k0 (A) is related
with a decreasing slope. by only one scalar value which is be abbreviated to s(t), hence
termed filter state.
3. MATHEMATICAL MODEL DEVELOPMENT t
αm · csol
In this section, a mathematical pressure drop model is de- s(t) ≡ 2 · · p(t) · dt [12]
ηg 0
veloped for a filter that leads to a characteristic function of the
permeability of the filter medium. This pressure drop model is The physical meaning of Equation (11) is that the evolution
based solely on the equations that comprise the cake filter model of the permeability on any area element A of the filter is solely
(Section 2) and the respective assumptions. determined by the evolution of the pressure drop over time. This
The time derivative of Equation (2) is is because the build up of the filter cake is the reason for the
1
changing permeability which, in turn, is merely determined by
d kc (t,A) dz(t, A) the filtration velocity and thus the pressure difference over the
= αm · [6]
dt dt filter.
PD METHOD FOR FILTER MEDIA CHARACTERIZATION 437
Equations (11) and (12) lead to an additive relation that de- to account for the substitution of the variable of integration by
scribes the permeability by two contributors, the initial perme- Equation (17):
ability k0−2 (A), only depending on the filter area and the filter
∞
state s(t) only depending on time. Thus, a separation of variables V̇ · ηg
[u + s(t)]− 2 d(u)
1
= [18]
is accomplished in the integrated form too. Atot p(t) u=0
k −2 (t, A) = k0−2 (A) + s(t) [13] The form of Equation (18) with a function as variable of
integration is called Riemann-Stieltjes integral. In this equation
In other words, the flow situation of the unloaded filter both p and s appear depending on time t. It is shown below
medium (Figure 1a) depends only upon the local domain. Based that the filter state s is treated as a parameter and therefore the
on that, the subsequent filter cake build up is only determined explicit time dependency can be omitted. The constant values
by the scalar filter state s(t), which is only time dependent. are abbreviated by a single factor pc :
So far the filter is considered on a scale resolving the inho-
mogeneities on the filter location A. However, to describe a filter V̇ · ηg
pc ≡ [19]
by a pressure drop model the entire filter must be considered. By Atot
integrating over all filter locations A, i.e., the entire filter area
Atot , in Equation (4) one obtains: which gives
∞
1 1
p(t) (u + s)− 2 d(u)
Atot Atot 1
= · [20]
v(t, A)dA = · k(t, A)dA [14] p pc
A=0 ηg A=0
0
converted to filter state s. Consequently a measured p(t) can [t(s), p(s)] for a sufficiently large number of different s-values.
be converted to exactly one corresponding p(s). These s-values are chosen to compute a pressure drop curve on
Equation (20) has the form of the generalized Stieltjes trans- a time range that is covering the entire measured pressure drop
formation. This integral transformation is treated by Hirschmann curve at a resolution superior to the experimental sampling rate.
and Widder (1955) who give an inversion formula for this prob- This computed pressure drop curve is linearly interpolated to
lem, i.e., a way to identify the distribution function (u) from each experimental measurement time value. Thus, for each ex-
the left-hand side, i.e., p(s). More importantly their inversion perimental point a computed pressure drop value is obtained
theory is based on uniqueness and the integral kernel in Equa- and the sum of the square errors can be calculated. The opti-
tion (20) is captured by that theory. Thus the inverse problem mization problem is an unconstrained nonlinear problem and
R
underlying Equation (20) is unambiguously determined. A given is solved with a commercially available code (Matlab Opti-
pressure drop curve p(s) has one and only one possible under- mization Toolbox). To increase the performance of the solver
lying permeability distribution function. the variables u i are scaled to vary around unity. The initial guess
The filter model outlined above is the core of the hence- supplied to the optimization algorithm is a vector of identical
forth termed the PD method: A measured pressure drop vs. time u i -values, i.e., a homogeneous PD.
profile of a filter is converted into a PD of the filter. This is It should be noted that the PD method uses only well-
accomplished via inversion of Equation (20). Since this equa- established parameters expressed by pc and tc (defined by Equa-
tion contains the filter state s as a parameter, the time is con- tions [19] and [21], respectively). Among these parameters only
verted to the filter state by using Equation (22), which is like- the specific cake resistance αm must be determined experimen-
wise uniquely invertible. Since no restrictions on the range of tally, because all other parameters that affect these two coeffi-
t and s were made, theoretically any arbitrary part of the left- cients are the design parameters of the filter plant and are thus
hand side function, i.e., p, can be chosen as input for the PD usually well known.
method. Since the measured pressure drop difference is in general
affected by a measurement error, the inversion of the mea-
sured p(s) function is in practice inconsistent, i.e., one cannot
Implementation obtain a PD that exactly fits every measurement point. How-
The available inversion theory for the Stieltjes transform ever, more importantly the accuracy of the inversion must be
makes use of arbitrary high derivatives of the p(s) function. examined. A detailed evaluation is performed and given else-
Thus the inversion theory does not straightforwardly lead to the where Koch (2008), since it would exceed the scope of this
computation of the distribution function. Practically numerical article.
methods succeed in solving the problem, which are discussed
in detail by Koch (2008). The hitherto continuous PD, (u),
is discretized. Equations (20) and (22) are rewritten in the dis- 5. EXPERIMENTAL
cretized formulation, whereby the integration is approximated Experimental pressure drop data, on which the PD method is
by the rectangle rule: applied, was gathered from two different laboratory-scale bag
filter plants. Both filter plants consisted of a two-screw feeder
1 1
m
that supplied a constant mass flow of dust to a dispersion noz-
(u i + s)− 2 i
1
= · [23]
p pc i=1 zle via a vibrating chute. Pressurized air dispersed the dust in
m
1
the nozzle. The dispersed dust was mixed with the gas stream,
1
t = tc · (u i + s) 2 − u i2 i [24] which was sucked through the filter plant by an induced draft
i=1 fan. The gas volume flow after the filter was recorded and con-
trolled to a certain set value via the frequency-controlled fan.
The PD (u) and the variable u are discretized with index i into The dust-laden gas entered the filter housing near the bottom. In
m intervals. In the approximation of the integral the frequency the filter housing three filter bags were mounted on wire cages.
distribution i is used, which will be defined as the discrete The bags were pervaded by the dust-laden gas from the outside
difference i = i − i−1 . The discretization of the cumula- to the inside. Dust particles were retained at the outer surface
tive distribution function is fixed with a constant i = m1 . of the filter bags. The clean gas flowed upwards inside the fil-
The PD is obtained via optimization with the ui ’s being the op- ter bags and was collected in the clean gas header. Due to the
timization variables. The optimization goal is the sum of square dust that accumulated on the filter bags, a filter cake formed and
errors of the difference of the measured and computed pressure the overall permeability of the filter decreased. As the fan kept
drop curves. the volumetric flow rate of the gas constant, the pressure drop
The optimization goal computes the functions p via Equa- through the filter increased. The filter was regenerated either af-
tion (23) and t via Equation (24) for a given set of optimiza- ter a certain pressure drop over the filter was reached or after
tion variables u i . The filter state s is hereby arbitrary, which a certain time interval for filtration had elapsed. Filter regener-
allows for the computation of a parametric pressure drop curve ation was carried out by a reverse air jet pulse. Each filter bag
PD METHOD FOR FILTER MEDIA CHARACTERIZATION 439
jet pulse unit to a single set volume flow V̇ , listed in Table 1, according to
Equation (26).
PDC fan V̇
clean gas
p = pexp · [26]
dust laden gas V̇exp
800 200
slope of the linear asymptote of the pressure drop curve as dis-
1
cussed below.
fl ow V˙ , m3 · h
The controlled gas volume flow changed slightly due the re- 600
sponse time of the control loop. To account for a slightly varying
gas volume flow the measured pressure drop pexp is corrected 400 100
TABLE 1 200 ∆p
Design data of laboratory scale bag filter plants V̇exp
0 0
Plant Atot ṁ c ηg αm V̇ − 0 50 100 150 200 250 300
time, s
# m2 kg s−1 Pa s m kg−1 m3 h−1
1 2.04 8.4 10−4 1.8 10−5 6.67 109 240 FIG. 3. Pressure drop and volume flow at filter start up (in order to provide a
more concise presentation the volume flow is displayed as floating mean value
2 0.53 1.5 10−5 2.0 10−5 — 40 with 20 seconds two sided window length).
440 M. KOCH AND G. KRAMMER
The pressure drop curve has a positive curvature for the initial 1250
short period of 15–20 seconds after dust dosing started. During
this period, the dust concentration in the filter housing increases
sure drop level is reached again and the next bag is cleaned in 0.4
sequence.
The PD method is applied to experimental data displayed
0.2
in Figure 3. The initial progressive pressure drop increase is PD
omitted and the remaining pressure drop data are used as input integral mean
for the PD method. The resulting PD (k0 ) is displayed in Figure 0
0 0.5 1 1.5 2 2.5
5 alongside its integral mean value, i.e., the apparent permeabil- k0, m
x 10
ity of the clean filter cloth. Note that the PD (k0 ) depending on
the permeability is directly obtained from (u), since k0 and u FIG. 5. PD determined for the pressure drop rise shown in Figure 3. The
are unambiguously linked by means of Equation (16). The clean shaded area corresponds to the integral mean value which is displayed as the
filter cloth exhibits a strong PD with about 10–15% of the filter dashed lined in addition.
PD METHOD FOR FILTER MEDIA CHARACTERIZATION 441
1200 550
∆p experimental
1000 500
pressure difference ∆p, Pa
PD could be different for the same filter medium but a different Dufrêche, J., Prat, M., Schmitz, P., and Sherwood J. D. (2002). On the Apparent
dust, which requires caution when trying to apply one PD to a Permeability of a Porous Layer Backed by a Perforated Plate, Chem. Engineer.
different system. Sci. 57: 2933–2944.
Duo, W., Kirkby, N. F., Seville, J. P. K., and Clift, R. (1997). Patchy Cleaning of
The PD of a filter medium can change during filter operation. Rigid Gas Filters—I. A Probabilistic Model, Chem. Engineer. Sci. 52: 141–
It is demonstrated that in a laboratory set-up this change of the 152.
PD can be observed and PDs determined from pressure drop Hirschmann, I. I., and Widder, D. V. (1955). The convolution transform. Prince-
data of industrial filter plants could be a useful tool to monitor ton University Press, Princeton, New Jersey.
the filtration characteristics over the life cycle of the filter bag. Hoff, D., Meyer, J., and Kasper, G. (2005). Influence of Filter Media Texture
on the Slope of the Differential Pressure Curve for Rigid Surface Filters at
High Temperatures, in International Conference & Exhibition for Filtration
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A∗ dimensionless location on the filter Area Load in a Jet Pulsed Filter by a Mechanistic Model. Powder Technol.
133: 134–146.
Adist cumulative filter area, m2 Koch, D., Seville, J., and Clift, R. (1996). Dust Cake Detachment from Gas
Atot total area of filter, m2 Filters. Powder Technol. 86: 21–29.
csol solid concentration of raw gas reaching the filter, Koch, M., Saleem, M., Pucher, P., and Krammer, G. (2007). Condition-
kg m3 ing of Filter Bags with Reactive CaO and Ca(OH)2 Dust in Flue Gas,
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m number of nodes for the discretized PD, − and Filter Medium Characterization. PhD thesis, Norwegian University of
ṁ c dust mass flow to filter, kg s−1 Science and Technology, Trondheim, Norway, available online.
pc pre-factor in Equation (20), Pa m Kozeny, J. (1927). Über die kapillare Leitung des Wassers im Boden, Sitz. Ber.
Akad. Wiss. Wien. Math. Nat. (Abt. IIa), 136a: 271–306.
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u abbreviation for k0−2 (Chapter 3), m−2 Process with a Flat-Type Fabric Filter. Advanced Powder Technol. 17(3):
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Saleem, M., Krammer, G., Rüther, M., and Bischof, H. (2005). Optical Mea-
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Abbreviations Strangert, S. (1978). Predicting Performance of Bag Filters. Filtration and Sep-
PD permeability distribution aration January/February: 42–48.
Hereby the constants pc and tc , defined by Equations (19) and By changing the order of integration on the left-hand side one
(21), respectively, are used to replace the coefficients that ap- obtains:
pear in Equation (12) originally. Rearranging Equation (A1)
gives: tc ∞ s
(u + s)− 2 ds d(u) = t
1
[A5]
2 0 0
pc tc 1 dt
= [A2]
2 p ds Evaluating the inner integral gives:
1 s
The pressure drop p can be expressed by Equation (20): ∞
tc
2 (u + s) 2 0 d(u) = t
∞
2 0
tc dt
(u + s)− 2 d(u) =
1
[A3]
2 0 ds Using the boundaries of s gives:
Integration via s from zero to s yields: ∞
1 1
s tc (u + s) 2 − (u + 0) 2 d(u) = t [A6]
∞
tc 0
(u + s)− d(u)ds = t
1
2 [A4]
2 0 0 which is equivalent to the time transformation Equation (22).