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Applied Thermal Engineering 51 (2013) 1098e1106

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Applied Thermal Engineering


journal homepage: www.elsevier.com/locate/apthermeng

Enhance heat dissipation for projection lamps by MWCNTs


nano-coating
Tun-Ping Teng a, Tun-Chien Teng b, *
a
Department of Industrial Education, National Taiwan Normal University, No. 162, Sec. 1, He-ping E. Rd., Da-an District, Taipei City 10610, Taiwan, ROC
b
Department of Mechatronic Technology, National Taiwan Normal University, No. 162, Sec. 1, He-ping E. Rd., Da-an District, Taipei City 10610, Taiwan, ROC

h i g h l i g h t s

< We prepared MWCNTs nano-coating and applied to heat dissipation for projection lamp.
< The temperature, power consuming and illumination of the fixture were evaluated.
< The internal temperature of the fixture adopting halogen lamps reduces 5.4% at most.
< The internal temperature of the fixture adopting LED lamps reduces 3.2% at most.
< The power consumption reduces 12.9% at most for LED lamps with MWCNTs nano-coating.

a r t i c l e i n f o a b s t r a c t

Article history: In this study, we used two-step synthesis method to prepare nano-coating containing multi-walled
Received 17 March 2012 carbon nanotubes (MWCNTs) of different concentrations and applied the MWCNTs to heat dissipation
Accepted 7 November 2012 for the projection lamp fixtures. We quantitatively coated the nano-coating on the inner surface of the
Available online 15 November 2012
housing of the fixture and evaluated its effects on the internal temperature, power consumption, and
luminous output of the fixture for different conditions. The results show that both concentration of the
Keywords:
MWCNT nano-coating and the projecting angle of the fixture affect the internal temperature and power
Heat dissipation
consumption. With the MWCNT nano-coating of concentration at 1.328 wt.% and the projecting angle of
Illumination
Multi-walled carbon nanotubes
0 , the internal temperature of the fixture adopting the halogen lamp and that adopting the LED lamp
Nano-coating reduce 5.4%  2.1% and 3.2%  2.1% at most, respectively; the power consumption reduces 12.9%  2.1% at
Power consumption most for the LED lamp; the luminous output has no significant difference for either the halogen or LED
lamp. This study demonstrates MWCNT Nano-coating has great feasibility for heat dissipation of the
lighting fixture. Further, this concept can also be applied to the cases requiring non-contact heat dissi-
pation. Therefore, this study can widely contributes to energy saving and carbon emission reduction.
Ó 2012 Elsevier Ltd. All rights reserved.

1. Introduction can be regarded as a CNT nanofluid with higher viscosity. Although


the concept of adding CNTs into the working fluid to improve the
Recently, the carbon nanotubes (CNTs) have been being con- resultant thermal conductivity is well known, but the related
cerned by many researchers in the nano-material fields. Since the experimental results of the resultant thermal conductivity have not
CNTs have excellent thermal conductivity and mechanical proper- been identical. The resultant thermal conductivity might be due to
ties [1], adding the CNTs into the traditional working fluid (CNT some factors such as aspect ratios, material, structure of CNTs,
nanofluid) [2e7], ceramic materials [8e11], polymers [12], paraffin suspension performance, dispersants, and the synthesis method for
[13], and thermal paste [14,15] to improve both thermal perfor- preparing the experimental sample of nanofluids.
mance and mechanical properties of the base material demon- Choi et al. [2] dispersed the multi-walled carbon nanotubes
strates many excellent results. The coating or paint added by CNTs (MWCNTs) with a mean diameter of 25 nm and a length of 50 mm
into oil. The experimental results demonstrated that the thermal
* Corresponding author. Department of Mechatronic Technology, National conductivity of the MWCNT nanofluid at 1.0 vol.% enhanced more
Taiwan Normal University, No. 162, Sec. 1, He-ping E. Rd., Da-an District, Taipei City than 160% as compared with the base fluid at room temperature. Xie
10610, Taiwan, ROC. Tel.: þ886 2 7734 3527; fax: þ886 2 2358 3074.
et al. [3] conducted the thermal conductivity experiments that
E-mail addresses: walter.teng@ntnu.edu.tw, tube.t5763@msa.hinet.net
(T.-C. Teng).
dispersed the CNTs in distilled water, ethylene glycol and decene.

1359-4311/$ e see front matter Ó 2012 Elsevier Ltd. All rights reserved.
http://dx.doi.org/10.1016/j.applthermaleng.2012.11.006
T.-P. Teng, T.-C. Teng / Applied Thermal Engineering 51 (2013) 1098e1106 1099

Nomenclature Subscripts
a ambient
$
q heat flux, W bs back surface
A area, m2 c convection
h heat transfer coefficient, W/m2  C ex external
Int intensity, counts i inner
k thermal conductivity, W/m  C in internal
L thickness, m o outer
lx illumination, lx r radiation
pc power consumption, W T total
R thermal resistance,  C/W or ratio w wall
Rs reflection, %
T temperature,  C

Experimental results indicated that at least up to 20% of the thermal a good suspension performance for a long period, the dispersants
conductivity as compared with the base fluid. Garg et al. [4] reported that generally have low thermal conductivity wrap the nano-
the enhancement of thermal conductivity about 3%e5% at 25  C for particles to lead increase of the contact resistance on the solide
the MWCNT nanofluid of 1.0 wt.% that was ultrasonicated for 20e liquid interface. Therefore, overdosing surfactant or dispersant
80 min. Chen et al. [5] prepared the MWCNT/ethylene glycol nano- will decrease the thermal conductivity of nanofluids.
fluid of 1.0 vol.% by a wetemechanical reaction without using From the above literature we can realize the CNTs can improve
surfactant or dispersant. The thermal conductivity of the MWCNT/ heat transfer in either the fluid or solid state if it is well dispersed. In
ethylene glycol nanofluid was 17.5% higher than the base fluid. Chen this study we tried to apply MWCNTs to heat dissipation for another
and Xie [6] adopted the wetemechanochemical reaction method to important practical case–lighting fixtures because of eco-
produce the single, double-walled carbon nanotubes (SWCNTs and consciousness. Recently, energy saving and carbon emission reduc-
DWCNTs) and MWCNTs. The enhancement of thermal conductivity tion is a very important topic. So-called ‘energy saving and carbon
was 15.6%, 14.2%, and 12.1% for the SWCNTs, DWCNTs, and MWCNTs emission reduction’ focuses on how to efficiently utilize energy, use
at 0.2 vol.%, respectively. Phuoc et al. [7] adopted the cationic chi- less fossil energy, and reduce carbon emission. In addition, energy
tosan as a dispersant to stabilize the MWCNT/water nanofluid. The saving and carbon emission reduction should also include extending
thermal conductivity was enhanced from 2.3% to 13% for the nano- the product lifetime to reduce the wasted material. The lighting
fluid containing the MWCNTs at 0.5 wt.% to 3 wt.%. industry is one of the world’s great industrial sectors. It sells annually
Although most research has demonstrated that the nanofluid about 20 billion lamps of the three major types: incandescent lamp,
containing CNTs has enhancement of the thermal conductivity as fluorescent lamp, and high intensity discharge lamp. Operating
compared with the base fluid, the effect of CNTs on coating needs to those lamps is estimated currently to consume over 2700 TW-h
be further studied. When the coating material containing nano- (nearly 20% of total global electricity production, or approximately
particles (called ‘nano-coating’ hereafter) is dried to become the 3% of total energy consumption) and thus to produce about 2000
solid state, some mechanisms that enhance the thermal conduc- Megatons of CO2 emission [25]. Therefore, how to improve luminous
tivity through the particle motion will disappear. Some studies efficiency to reduce lighting energy consumption is a very important
demonstrated that adding CNTs in solid materials could enhance the task. Regarding the above concern, the light emitting diode (LED)
thermal conductivity of the base material [8,10,12,15], in which lighting is expected as a potential replacement for the traditional
Biercuk et al. [12] pointed that adding 1 vol.% SWCNTs to epoxy could lamp (especially for the incandescent lamp) due to its advantages
improve its thermal conductivity up to 125%. In contrast, some such as long lifetime, energy efficiency, wide range of colors, low-
studies showed that adding CNTs into the solid materials did not voltage power supply, and environmental compatibility [26,27].
enhance the thermal conductivity of the base materials [11,16,17]. Particularly, the development of LED technology has driven effi-
The main reasons are due to some factors such as interface thermal ciency and luminous output of LED to rise exponentially. For
resistance between the base materials and CNTs, increased porosity, example, a laboratory prototype LED achieving 208 lumens per watt
inhomogeneous distribution, agglomeration of CNTs, and incom- at room temperature was also announced in 2010 [28,29]. Therefore,
plete consolidation processing [11]. Therefore, the nanoparticles LED has prospect of providing the majority of light sources by 2035
must be uniformly dispersed into coating liquid, and the coating film [30]. Despite the above advantages of LED, LED still has the serious
after drying must be closely integrated with the coating substrate. problem that efficiency and lifetime falls sharply with heat rising to
Generally, the ultrasonic vibrator, electromagnetic stirrer, be resolved [31,32]. So, how to manage heat dissipation for LED is
homogenizer, and other physical dispersion are most commonly a study-worthy topic; consequently many related researches have
used to mix nano-materials into base fluid for better suspension been proposed [33e37]. In this study we selected a projection lamp
[4,18,19]. However, it is difficult for these physical dispersion fixture as the experiment subject, and this fixture can adopt either
methods to resolve agglomeration problem resulted from the van the LED lamp or halogen lamp. We coated the inner housing wall of
der Waals interaction forces, non-reactive surface properties, very the fixture with the MWCNT nano-coating to improve its heat
large specific surface areas, and aspect ratios of CNTs [7,20e22]. dissipation and then investigated the effect on both the internal
Therefore, many researchers add the surfactant or dispersant in temperature and power consumption of the fixture that adopted the
order to improve dispersion in nanofluids. The commonly used LED lamp. In addition, since the traditional light sources still play
dispersant contains nitric/sulfuric acid mixture, potassium a role in the immediate future through developments in the design
hydroxide group [5,23], and various surfactants such as sodium and control of lighting installations to provide substantial energy
dodecylbenzene sulphonate (SDBS), sodium dodecyl sulfate (SDS), saving opportunities [38], the projection lamp fixture adopting
and gum Arabic (GA) [18,24]. Although adding dispersants can halogen lamps was also tested as comparison group in this
improve dispersion of nano-materials in the base fluid to maintain experiment.
1100 T.-P. Teng, T.-C. Teng / Applied Thermal Engineering 51 (2013) 1098e1106

2. Theories for heat transfer value, T2 closer to T1 represents the lower total thermal resistance
between space A and B.
Fig. 1 shows the heat transfer process from space A to B based on According to the above-mentioned concept of heat transfer,
$
the concept of steady-state heat transfer, the heat flux (ðqT Þ) can be reducing the thermal resistance can increase the heat transfer
expressed as: performance. The thermal resistance of radiation is mainly deter-
mined by both the shape factor and surface optical properties of
$
qT ¼ hT AðT1  T2 Þ ¼ ðT1  T2 Þ=RT ; (1) materials; the thermal resistance of convection depends mainly on
both the airflow rate and surface properties; thermal conductivity
where hT is total heat transfer coefficient; A is area of heat transfer; is determined by the thermal conductivity of the material itself.
T is temperature; RT is total thermal resistance; the subscripts 1 and Therefore, using the higher absorption coating or anti-reflective
2 refer to space A and B, respectively. In the process of heat transfer, structure on the wall can reduce the thermal resistance of radia-
the relationship of heat transfer coefficient (h) and the thermal tion; increasing the airflow vents can reduce the convective
resistance (R) in the conduction, convection, and radiation are thermal resistance; using the material with high thermal conduc-
sequentially expressed as: tivity to make the wall can effectively reduce the thermal resistance
of heat conduction. Similarly, coating a film containing the
Rw ¼ ð1=hw AÞ ¼ ðL=kAÞ; (2) MWCNTs that has both high thermal conductivity and high optical
absorption properties on the either inner or outer surface of
Rc ¼ ð1=hc AÞ; (3) a closed or semi-enclosed lampshade can also both enhance the
heat dissipation performance of the lighting fixture and extend
lifetime of the lamp.
Rr ¼ ð1=hr AÞ; (4)

where the subscripts w, c, and r refer to conduction, convection, 3. Preparation of MWCNT nano-coating and experimental
and radiation, respectively. design
The convection and radiation occur simultaneously at a surface,
and both the thermal resistance of convection and radiation can be 3.1. Preparation of test samples
combined into a single thermal resistance. The total thermal
resistance based on the concept of electrical series and parallel Fig. 2 and Fig. 3 are the photographs of Multi-walled carbon
resistance can be expressed as follows: nanotubes (MWCNTs, Cheap Tubes Inc.) through the high-
resolution field emission scanning electron microscope (HR-
   
RT ¼ R1;c ==R1;r þ Rw þ R2;c ==R2;r : (5) FESEM, S4800, Hitachi) and transmission electron microscope
(TEM, H-7100, Hitachi), respectively. According to the specification
The heat flux is constant when the heat transfer from space A to provided by the manufacturer, the MWCNTs have an outside
B under steady state conditions, and then the Eq. (1) can be diameter of 20e30 nm, inside diameter of 5e10 nm, length of 10e
rewritten as follows: 30 mm, average density of 2.1 g/cm3, and thermal conductivity of
$    about 300e400 W/mK. As we can see from those figures, the
qT ¼ ðT1  Ts1 Þ= R1;c ==R1;r ¼ ½ðTs1  Ts2 Þ=Rw  MWCNTs aggregate, and their primary outside diameter is
  
¼ ðTs2  T2 Þ= R2;c ==R2;r : (6) approximately in line with the specification.
We used the MWCNTs/water nanofluid produced by two-step
In the Eq. (6), we can find that the smaller temperature differ- synthesis method as the dilute liquid. First, we added 0.2 wt.% of
ence represents the lower thermal resistance of the interface when cationic dispersant (water-soluble chitosan) into distilled water as
the heat flux is constant. In contrast, when T1 keeps at a constant the base liquid in order to obtain good dispersion performance for
the MWCNTs/water nanofluid. Chitosan is widely used in medicine,
agriculture, chemical, and food processing areas without causing

Fig. 1. The diagram of heat transfer process. Fig. 2. HR-FESEM images of MWCNTs.
T.-P. Teng, T.-C. Teng / Applied Thermal Engineering 51 (2013) 1098e1106 1101

(80  80  0.3 mm) to form the sample 2, 3, and 4 under the spray
pressure at 2.0 kg/cm2. After each spraying process was finished,
the samples were dried in an oven for 3 h at 50  C. We measured
the thickness of the coating films on the samples by thickness
meter (LZ-370, KETT) at accuracy of 2%, and the thickness
measured 70  5 mm. We also measured reflection spectra of each
sample by VIS-NIR spectrometer (BRC112E, B&W) at a resolution
of 2 nm.

3.2. Design and process of heat dissipation experiment

In order to test the heat transfer performance of the galvanized


steel plate coated with the MWCNTs, the test configuration was
setup as shown in Fig. 4. In this test, the coated surface (front
surface) of the experimental sample facing the hot plate (PC-420D,
Corning) was heated at a fixed distance (250 mm) away from the
hot plate at the different heating temperatures (60, 80, 100, 120,
and 140  C), and two thermocouples were attached on the back
surface of the sample to measure the temperature. Thus, the
temperature of back surface of the test samples can determine the
heat transfer performance. The accuracy of the K-type thermo-
couple is 0.1  C.
In order to investigate the performance of the MWCNT nano-
coating applied to heat dissipation for the projection lamp
Fig. 3. TEM images of MWCNTs. fixture, we implemented the heat dissipation performance exper-
iment on the projection lamp fixture. Fig. 5 shows the structure of
the projection lamp fixture in this study. This projection lamp
environmental pollution due to its non-toxic and biodegradable
fixture contains a cylindrical housing with vents thereon, vents (the
features, so this study used the water-soluble chitosan as a disper-
lower and upper), a lamp, and a holder that can pose the cylindrical
sant for the MWCNTs/water nanofluid [7,19]. Second, we gradually
housing at different projecting angle. The projecting angle affects
added the MWCNTs into the base liquid step by step and up to the
the heat dissipation of the vents due to direction change of the
needed weight through a precision electronic balance (XS125A,
airflow in the vents. In order to investigate the effects of the
Precisa) at a precision of 0.1 mg. Thirdly, in order to keep the
MWCNT nano-coating and projecting angle (0 or 90 ) on heat
nanoparticle with stable suspension in the base liquid, we alter-
dissipation of the fixture, we attached the K-type thermocouple
nately used an electromagnetic agitation (PC-420D, Corning),
with accuracy of 0.1  C on both the lamp socket and outer surface
homogenizer (T25 digital, IKA), and ultrasonic vibrator (D400H,
of the housing by high thermal conductivity adhesive (plastic steel
TOHAMA) for about 3 h to disperse the MWCNTs. The prepared
epoxy 3344, PowerBon), and connected the thermocouple with
MWCNTs/water nanofluid had three weight fractions (1.0, 2.0,
a data logger (TRM-20, TOHO) to measure the temperature when
4.0 wt.%).
the lamp was turned on. Before the experiment was implemented,
Next, the MWCNT nano-coating was produced. First, we used
we carefully selected three fixtures, three halogen lamps, and three
the trial and error method to repeatedly test the optimal amount of
LED lamps for prior test to make sure that the difference in illu-
solvent (MWCNTs/water nanofluid) to dilute the bulk material for
mination, power consumption, and internal temperature between
easy spray, and thus obtained the optimal dilution of volume ratio
the three fixtures with the lamp of the same kind is within 2.0%.
at 40 vol.%. The ingredients of the different kinds of the dilution
solvent are listed in Table 1. The bulk material is water-based paint
(National Ltd. Co., Taiwan). The density of the bulk material is
1340 kg/m3, and its main ingredient is an acrylic polymer. The
MWCNT nano-coating was dispersed several times by a homoge-
nizer, electromagnetic stirrer, and ultrasonic vibrator in order to
make it easy to be sprayed.
We sprayed the MWCNT nano-coating of each different
concentration twice times on each galvanized steel plate

Table 1
Preparation parameters of MWCNTs nano-coating.

Sample no. Sample 1 Sample Sample Sample


2 3 4
Density of water-based paint Non-coating 1340
(kg/m3)
MWCNTs/water nanofluid 1.0 2.0 4.0
(wt.%)
Dilution of volume ratio 40
(vol.%)
MWCNTs concentration in 0.332 0.664 1.328
coating (wt.%)
Fig. 4. Setup to test heat transfer performance for MWCNTs coating.
1102 T.-P. Teng, T.-C. Teng / Applied Thermal Engineering 51 (2013) 1098e1106

housing was coated by the paint containing the MWCNTs according


to the procedure same as the above-mentioned background
experiment. Finally, we compared the difference in the tempera-
ture, illumination, and power consumption of the projection lamp
fixtures between those with and without the MWCNT nano-coating
in order to investigate the effects of the MWCNT nano-coating on
heat dissipation and lighting performance. Furthermore, In order to
reduce experimental deviation, the environmental temperature
was controlled at 25  0.5  C during the experiments.

3.3. Uncertainty and data analysis

The uncertainty of the results of this experiment were deter-


mined by measuring the deviation in the parameters, including the
illumination, power consumption, and temperature. Because we
mainly evaluated the difference between the same fixture without
coating and with coating, the deviation between the fixtures had
little impact on evaluation. In the heat dissipation experiment for
the projection lamp; the illumination (lx) was determined from
readings of the illuminometer; the power consumption (pc) was
measured by the digital power meter; the internal (Tin) and
external (Tex) temperature was measured by the data logger; the
ambient temperature (Ta) was controlled by the temperature
controller of DC inverter air conditioner. The uncertainty of illu-
mination, power consumption, and temperature in the heat dissi-
pation experiment for the projection lamp experiment can be
expressed as Eqs. (7)e(9), respectively.
qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
um;lx ¼ ðDlx=lxÞ2 þðDTa =Ta Þ2 (7)

qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
um;pc ¼ ðDpc=pcÞ2 þðDTa =Ta Þ2 (8)

qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
um;T ¼ ðDT=TÞ2 þðDTa =Ta Þ2 (9)
Fig. 5. The structure of projection lamp fixture at different projecting angle. (a) 90 ,
(b) 0 . The accuracy of the illuminometer is within 3.0%. The accuracy
of the digital power meter is within 0.35%. The accuracy of the
First, we turned on the three fixtures with a halogen lamp (Decostar thermocouple for internal and external temperature of the
51/50W/12V/38deg., OSRAM) for 70 min as background experi- projection lamp is within 0.1  C. The accuracy of the temperature
ment, and then replaced the lamp with a LED lamp (MR-16/3.5W/ controller of DC inverter air conditioner for ambient temperature is
12V/50deg., China Electric mfg. Corporation) for the same back- within 0.5  C. Therefore, the uncertainty of the illumination,
ground experiment. The temperature data were averages of the power consumption, and temperature experiment is within 3.6%,
data measured in the last 10 min of the background experiment. 2.1%, and 2.1%, respectively.
When the illuminating time reached 60 min, we started to measure
both the illumination and power consumption of each fixture by an 3.4. Data analysis
illuminometer (TES-1336A, TES) with accuracy of 3.0% and
a digital power meter (WT230, Yokogawa) with accuracy of 0.35% The measurement data of heat dissipation performance, illu-
for different lighting sources (halogen lamps and LED lamps) and mination, and power consumption for the lamp fixture with
projecting angles (0 and 90 ) in order to obtain the differences in uncoated housing are referred as baseline values (Db), and the
power consumption and illumination on the surface at a fixed measurement data for the lamp fixture with housing coated by
distance below the fixture. The data of illumination and power paint containing the MWCNTs are marked as Dc. For explicit
consumption were averages of the ten measurements with an investigation, the experimental data Dc were compared with Db.
interval of 1 min during the last 10 min in the experiment. Next, the The differences between Dc and Db are presented as proportions (R)
inner surfaces of the cylindrical housing of the three fixtures were and are expressed as follows:
coated with the paint containing the MWCNTs of three different
concentrations at 0.332, 0.664, and 1.328 wt.%, respectively. In
R ¼ ðDc =Db Þ  100%: (10)
order to obtain the uniform coating on the inner surface and reduce
the thickness differences between the samples, we fixed the
cylindrical housing horizontally and concentrically at a motor shaft 4. Results and discussion
to let the housing rotate at 600 rpm for 20 min to make the coated
paint dry and uniform after the paint was quantitatively brush Fig. 6 shows the reflection spectra of the samples. The sample 1
(1.0 ml) by quantitative dropper and rubber spatula. Then, the is bare galvanized steel plate without coating, sample 2e4 are
samples were dried in the oven at 50  C. Next, we conducted the coated by the paint containing the MWCNTs of 0.332, 0.664, and
heat dissipation experiment on the projection lamp fixtures whose 1.328 wt.%, respectively. In the Fig. 6, we can find that adding
T.-P. Teng, T.-C. Teng / Applied Thermal Engineering 51 (2013) 1098e1106 1103

Fig. 6. Reflection spectra of the test samples. Fig. 8. Internal temperature trends of halogen lamp at different projecting angles.

the MWCNTs can reduce the reflectivity within UVeNIR band because the MWCNTs have both excellent optical absorption and
(350e950 nm), and the reflectivity decreases with increase in high thermal conductivity (about 300e400 W/mK) to reduce
concentration of the MWCNTs. This phenomenon is mainly because thermal resistance in both radiation and conduction. As seen from
the MWCNTs have excellent optical absorption within UVeNIR Fig. 6, MWCNT nano-coating has high optical absorption such that
band. However, when concentration of the MWCNTs exceed the thermal resistance in radiation can be reduced. Further, because
above 0.664 wt.%, there is no significant difference in reflectivity the overall thermal conductivity of the mixture depends on the
because absorption reaches saturation. thermal conductivity of each ingredient, adding the material with
Fig. 7 shows the heat transfer performance of the samples. In high thermal conductivity into the bulk material can increase the
Fig. 7, we can find that adding the MWCNTs can increase the overall thermal conductivity [39,40]. Therefore, the total thermal
temperature of the back surface of the sample, and the temperature resistance also reduces when the thermal resistance decreases in
increases with increase in concentration of the MWCNTs. For the both radiation and heat conduction.
same heating temperature of the hot plate, the higher back surface Fig. 8 and Fig. 10 show the temperature of the lamp socket
temperature means that there is greater heat flux through the (called ‘internal temperature’ hereafter) of the lamp fixtures at
sample, and the sample has lower thermal resistance; consequently different projecting angle in the background test, and the related
providing better heat dissipation. This phenomenon is mainly data can be referred to Table 2. Figs. 9 and 11 show the temperature

Fig. 7. Heat transfer performance of the samples. Fig. 9. External temperature trends of halogen lamp at different projecting angles.
1104 T.-P. Teng, T.-C. Teng / Applied Thermal Engineering 51 (2013) 1098e1106

concentration at 0.332, 0.664, and 1.328 wt.%, respectively are


called ‘fixture 1’, ‘fixture 2’, and ‘fixture 3’, respectively. Fig. 12
shows the ratio of internal temperature of the fixture with coated
housing to that of the corresponding fixture with uncoated
housing. In Fig. 12, we can find that there is more significant effect
for the fixtures at a projecting angle of 0 . For the halogen lamp,
little effect is observed at a projecting angle of 90 . However, for
the fixtures at a projecting angle of 0 , the internal temperature of
the fixtures with inner housing wall coated by paint containing the
MWCNTs of concentration at 0.332, 0.664 wt.% (fixture 1 and
fixture 2) increases instead. It is because the bulk material of the
paint has higher thermal resistance such that the total thermal
resistance of the paint is still higher when the added the MWCNTs
are fewer. When concentration of the added MWCNTs reaches
1.328 wt.%, the internal temperature is reduced 5.4%  2.1% as
compared with the uncoated case. For the LED lamp, similarly, little
effect is observed at projecting angle of 90 . For the fixtures at
a projecting angle of 0 , the internal temperature is reduced
3.2%  2.1% for the fixture with inner housing wall coated by paint
containing the MWCNTs of concentration at 1.328 wt.%. For both
the halogen and LED lamps at a projecting angle of 0 , the internal
temperature decreases with increase in concentration of the
Fig. 10. Internal temperature trends of LED lamp at different projecting angles. MWCNTs.
Similarly, in order to investigate the effects of the MWCNT nano-
coating on power consumption of the fixtures, the power
of the outer housing surface (called ‘external temperature’ here- consumption of each fixture with coated housing is compared with
after) of the lamp fixtures at different projecting angle in the that of the same fixture before its housing is coated. Fig. 13 shows
background test. As we can see from those figures, both the internal the ratio of power consumption of the fixture with coated housing
temperature and external temperature at projecting angle of 90 is to that of the corresponding fixture with uncoated housing. In
higher than that at the projecting angle of 0 . This phenomenon can Fig. 13, we can find that there is no effect of the MWCNT nano-
be explained as follows (please also refer to Fig. 5): at the projecting coating on power consumption of the fixtures for the halogen
angle of 90 , the cold air enters into the bottom vents and the lamp. In fact, the power consumption of halogen lamp is affected by
heated air discharges from the top vents according to the principle temperature of the filament. In order to stabilize the power
of heat convection. Thus, the heated air flows by the lamp socket consumption of the lamp, the resistance of the filament is designed
and heats it; major portion of the heat generated by the lamp is to increase with the increase in temperature. For such design, when
transferred by convection, and minor portion is dissipated through the temperature of the filament increases due to increase in dissi-
the housing wall. In contrast, at the projecting angle of 0 , most of pation power, the resistance of the filament also increases such that
the heated air does not flow by the lamp socket, so the internal the power consumption is suppressed. In contrast, when the
temperature is lower. Furthermore, at the projecting angle of 0 , the temperature of the filament decreases due to decrease in dissipa-
housing wall provides greater effective heat transfer area, and the tion power, the resistance of the filament decreases such that
heated air easily discharge from the vents on the housing wall, so power consumption increases. It should be noted that the luminous
the external temperature is also lower. From Figs. 8 and 9, we can efficiency decreases as the temperature of the filament decreases
find that the difference of internal and external temperature according to the blackbody irradiation principle. Therefore,
between 90 and 0 at 60 min after the halogen lamp was turned on although the lower temperature benefits the lifetime of the fila-
is about 28  C and 10  C, respectively. From Figs. 10 and 11, we can ment, the temperature is still set at the optimal regarding the
find that the difference of internal and external temperature luminous efficiency [41e43]. For the above reasons, we just cool
between 90 and 0 at 60 min after the LED lamp was turned on is down the local temperature of the lamp socket instead of the fila-
about 3  C and 1.5  C, respectively. ment in this study. For the halogen lamp, just little portion of the
In order to investigate the effects of the MWCNT nano-coating heat generated by the filament dissipates through the lamp socket,
on the internal temperature of the fixtures, the temperature of so cooling down the local temperature of the lamp socket has very
each fixture with coated housing is compared with that of the same little impact on the filament temperature. It can be proved by
fixture before its housing is coated. The three fixtures with inner checking if the output spectra of the lamp changes. In this study,
housing wall coated by paint containing the MWCNTs of the output spectra were monitored and had very little variation

Table 2
Experimental results of initial condition for baseline.

Test parameters Deg. Halogen RSD LED RSD


lamp lamp
Illumination (lx) 90 9980 9980 9760 1.05% 556 554 545 0.87%
0 10,060 10,090 9860 1.02% 554 535 533 1.75%
Internal temperature ( C) 90 173.15 174.91 170.19 1.13% 51.81 52.89 50.96 1.52%
0 146.78 151.41 153.18 1.79% 48.69 49.48 48.03 1.22%
Power consumption (W) 90 39.60 40.08 38.64 1.52% 3.88 3.88 3.88 0.00%
0 40.08 40.56 39.12 1.50% 3.92 3.90 3.90 0.24%

Note: Relative standard deviation (RSD) ¼ (standard deviation/mean)  100%.


T.-P. Teng, T.-C. Teng / Applied Thermal Engineering 51 (2013) 1098e1106 1105

Fig. 11. External temperature trends of LED lamp at different projecting angles.

during the experiment. Since the filament temperature was not Fig. 13. Power consumption ratio of fixtures at different projecting angles.
affected in the experiment, the power consumption does not
change. In contrast, for the LED lamp, Fig. 13 shows the MWCNT
nano-coating has some effect on the power consumption. Espe- can also reduce the junction temperature of LED chip. Further, since
cially for the higher concentration of the MWCNT nano-coating, the LED needs DC electricity power, the related rectifier electronics are
power consumption reduces 12.9%  2.1% at most. It is mainly due integrated on the bottom of the LED lamp. Thus, lower temperature
to both the characteristic of LED chip and rectifier electronics of the lamp socket also can reduce the power consumption and
integrated in the LED lamp. The junction temperature quite impacts benefit the lifetime of the electronics. Based on the above reasons,
the luminous efficiency and lifetime of the LED chip; the luminous the MWCNT nano-coating has more obvious effect on power
efficiency and lifetime exponentially decreases as the junction consumption of the LED lamps.
temperature increases. Because LED is a ‘cold light’ source, the most Similarly, in order to investigate the effects of the MWCNT nano-
heat generated from the LED chip is conducted out through the coating on the illumination, the illumination of each fixture with
substrate. Thus, cooling down the temperature of the lamp socket coated housing is compared with that of the same fixture before its

Fig. 12. Internal temperature ratio of fixtures at different projecting angles. Fig. 14. Illumination ratio of fixtures at different projecting angles.
1106 T.-P. Teng, T.-C. Teng / Applied Thermal Engineering 51 (2013) 1098e1106

housing is coated. Fig. 14 shows the ratio of illumination of the [10] R. Sivakumar, S.Q. Guo, T. Nishimura, Y. Kagawa, Thermal conductivity in
multi-wall carbon nanotube/silica-based nanocomposites, Scr. Mater. 56
fixture with coated housing to that of the corresponding fixture
(2007) 265e268.
with uncoated housing. In Fig. 14, we can find that there is little of [11] K. Chu, Q. Wu, C. Jia, X. Liang, J. Nie, W. Tian, G. Gai, H. Guo, Fabrication and
the MWCNT nano-coating on illumination of the fixtures for either effective thermal conductivity of multi-walled carbon nanotubes reinforced
the halogen lamp or LED lamp. The difference in the experiment Cu matrix composites for heat sink applications, Compos. Sci. Technol. 70
(2010) 298e304.
data is within the deviation of the illumination experiment (3.6%). [12] M.J. Biercuk, M.C. Llaguno, M. Radosavljevic, J.K. Hyun, A.T. Johnson, Carbon
In this study, the above results demonstrate that the MWCNT nanotube composites for thermal management, Appl. Phys. Lett. 80 (2002)
nano-coating can indeed reduce the internal temperature of the 2767e2769.
[13] T.P. Teng, B.G. Lin, Y.Y. Yeh, Characterization of heat storage by
fixtures and reduce the power consumption (for LED lamps) while nanocomposite-enhanced phase change materials, Adv. Mater. Res. 287e290
maintains the same luminous output. Therefore, this study will (2011) 1448e1455.
contribute to lifetime of the components, energy saving and carbon [14] D.D.L. Chung, Materials for thermal conduction, Appl. Therm. Eng. 21 (2001)
1593e1605.
emission reduction. [15] Y. Xu, C.K. Leong, D.D.L. Chung, Carbon nanotube thermal pastes for improving
thermal contacts, J. Electron. Mater. 36 (2007) 1181e1187.
5. Conclusions [16] C. Kim, B. Lim, B. Kim, U. Shim, S. Oh, B. Sung, J. Choi, J. Ki, S. Baik,
Strengthening of copper matrix composites by nickel-coated single-
In this study, we quantitatively painted the inner housing wall of walled carbon nanotube reinforcements, Synth. Met. 159 (2009)
424e429.
the projecting lamp fixtures with the MWCNT nano-coating of [17] C.W. Nan, R. Birringer, Determining the Kapitza resistance and the
different concentration in order to reduce the internal temperature thermal conductivity of polycrystals: a simple model, Phys. Rev. B 57
of the fixtures for the purpose of both extending the lifetime of the (1998) 8264e8268.
[18] Y. Ding, H. Alias, D. Wen, R.A. Williams, Heat transfer of aqueous suspensions
components and saving energy. The experimental results show that of carbon nanotubes (CNT nanofluids), Int. J. Heat Mass. Transf. 49 (2006)
the internal temperature reduces 5.4%  2.1% (for the halogen 240e250.
lamp) and 3.2%  2.1% (for the LED lamp) at most for the fixture [19] Y.H. Hung, T.P. Teng, T.C. Teng, J.H. Chen, Assessment of heat dissipation
performance for nanofluid, Appl. Therm. Eng. 32 (2012) 132e140.
with housing coated by the MWCNT nano-coating of 1.328 wt.% at [20] L.A. Girifalco, M. Hodak, R.S. Lee, Carbon nanotubes, buckyballs, ropes, and
the projecting angle of 0 . The power consumption reduces a universal graphic potential, Phys. Rev. B 62 (2000) 13104e13110.
12.9%  2.1% (for the LED lamp) at most for the fixture with housing [21] T. Lin, V. Bajpai, T. Ji, L. Dai, Chemistry of carbon nanotubes, Aust. J. Chem. 56
(2003) 635e651.
coated by the MWCNT nano-coating of 1.328 wt.% at the projecting
[22] C. Park, Z. Ounaies, K.A. Watson, R.E. Crooks, J.J. Smith, S.E. Lowther, Disper-
angle of 0 . The MWCNT nano-coating has no effect on luminous sion of single wall carbon nanotubes by in situ polymerization under soni-
output for either the halogen lamp or LED lamp. This study cation, Chem. Phys. Lett. 364 (2002) 303e308.
demonstrates that the MWCNT nano-coating has high feasibility in [23] G.H. Ko, K. Heo, K. Lee, D.S. Kim, C. Kim, Y. Sohn, M. Choi, An experimental
study on the pressure drop of nanofluids containing carbon nanotubes in
heat dissipation for lighting fixtures, which benefits the lifetime of a horizontal tube, Int. J. Heat Mass. Transf. 50 (2007) 4749e4753.
the related components. Further, the MWCNTs can also extend to [24] L. Jiang, L. Gao, J. Sun, Production of aqueous colloidal dispersions of carbon
be applied to the cases requiring non-contact heat dissipation. nanotubes, J. Colloid Interface Sci. 260 (2003) 89e94.
[25] OECDJIEA, Light’s Labour’s Lost: Policies for Energy-efficient Lighting. Paris
Therefore, this study can widely contribute to energy saving and Cedex, France (2006).
carbon emission reduction. [26] R. Devonshire, The competitive technology environment for LED lighting,
J. Light Vis. Environ. 32 (2008) 275e287.
[27] N. Zheludev, The life and times of the LED- a 100-year history, Nat. Photonics
Acknowledgements 1 (2007) 189e192.
[28] Nature Photonics Editorial, Haitz’s law, Nat. Photonics 1 (2007) 23.
The authors would like to thank National Science Council of the [29] CREE, Cree breaks 200 lumen per watt efficacy barrier (Press release), CREE,
Durham, N.C, 2010.
Republic of China, Taiwan for their financial support to this research [30] M. Richards, D. Carter, Good lighting with less energy: where next? Lighting
under contract no.: NSC-100-2221-E-003-029 and NSC-100-2221- Res. Technol. 41 (2009) 285e286.
E-003-015, respectively. [31] A.A. Efremov, N.I. Bochkareva, R.I. Gorbunov, D.A. Lavrinovich, Y.T. Rebane,
D.V. Tarkhin, Y.G. Shreter, Effect of the joule heating on the quantum effi-
ciency and choice of thermal conditions for high-power blue InGaN/GaN LEDs,
References Semiconductors 40 (2006) 605e610.
[32] S.L. Chuang, A. Ishibashi, S. Kijima, N. Nakayama, M. Ukita, S. Taniguchi,
[1] S.M.S. Murshed, K.C. Leong, C. Yang, Thermophysical and electrokinetic Kinetic model for degradation of light-emitting diodes, IEEE J. Quantum
properties of nanofluids e a critical review, Appl. Therm. Eng. 28 (2008) Electron. 33 (1997) 970e979.
2109e2125. [33] Philips and Lumileds Co. Ltd., Understanding Power LED Lifetime Analysis, in:
[2] S.U.S. Choi, Z.G. Zang, W. Yu, F.E. Lookwood, E.A. Grulke, Anomalous thermal Technology White Paper, Philips and Lumileds Co. Ltd., 2007.
conductivity enhancement in nanutube suspension, Appl. Phys. Lett. 79 (2001) [34] E. Hong, N. Narendran, A method for projecting useful life of LED lighting
2252e2254. systems, 3rd International Conference on Solid State Lighting, Proc. SPIE 5187
[3] H. Xie, H. Lee, W. Youn, M. Choi, Nanofluids containing multiwalled carbon (2004) 93e99.
nanotubes and their enhanced thermal conductivities, J. Appl. Phys. 94 (2003) [35] J. Hu, L. Yang, M.W. Shin, Mechanism and thermal effect of delamination in
4967e4971. light-emitting diode packages, Microelectron. J. 38 (2007) 157e163.
[4] P. Garg, J.L. Alvarado, C. Marsh, T.A. Carlson, D.A. Kessler, K. Annamalai, An [36] M. Bürmen, F. Pernus, B. Likar, Prediction of intensity and color degradation of
experimental study on the effect of ultrasonication on viscosity and heat LEDs, Proc. SPIE 6486 (2007) 64860M1e10.
transfer performance of multi-wall carbon nanotube-based aqueous nano- [37] J.H. Choi, M.W. Shin, Thermal investigation of LED lighting module, Micro-
fluids, Int. J. Heat Mass Transf. 52 (2009) 5090e5101. electron. Reliab. (2011). http://dx.doi.org/10.1016/j.microrel.2011.04.009.
[5] L. Chen, H. Xie, Y. Li, W. Yu, Nanofluids containing carbon nanotubes treated [38] D. Loe, Energy efficiency in lighting e considerations and possibilities,
by mechanochemical reaction, Thermochim. Acta 477 (2008) 21e24. Lighting Res. Technol. 41 (2009) 209e218.
[6] L. Chen, H. Xie, Surfactant-free nanofluids containing double- and single- [39] J.C. Maxwell, A Treatise on Electricity and Magnetism, third ed., vol. 1, Clar-
walled carbon nanotubes functionalized by a wet-mechanochemical reac- endon, Oxford, 1904.
tion, Thermochim. Acta 497 (2010) 67e71. [40] R.L. Hamilton, O.K. Crosser, Thermal conductivity of heterogeneous two
[7] T.X. Phuoc, M. Massoudi, R.H. Chen, Viscosity and thermal conductivity of component systems, I&EC Fundam. 1 (1962) 182e191.
nanofluids containing multi-walled carbon nanotubes stabilized by chitosan, [41] S. Garbe, S. Hanloh, Growth of potassium-filled bubbles in doped tungsten and
Int. J. Therm. Sci. 50 (2011) 12e18. its relation to hot spot development and intergranular fracture, Philips J. Res.
[8] C.H. Liu, H. Huang, Y. Wu, S.S. Fan, Thermal conductivity improvement of silicone 38 (1983) 248e262.
elastomer with carbon nanotube loading, Appl. Phys. Lett. 84 (2004) 4248e4250. [42] Publication Number TP-110Incandescent Lamps, General Electric Company,
[9] G.D. Zhan, J.D. Kuntz, J. Wan, A.K. Mukherjee, Single-wall carbon nanotubes as Nela Park, Cleveland, OH, 1964.
attractive toughening agents in alumina-based nanocomposites, Nat. Mater. 2 [43] R. Kane, Heinz Sell Revolution in Lamps: A Chronicle of 50 Years of Progress,
(2003) 38e42. second ed., The Fairmont Press, Inc, 2001.

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