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t
N. Ryzhanova1,2 , A. Vedyayev1,2 , A. Pertsova2 , B. Dieny1
1
Abstra t
I. INTRODUCTION
Re
ently there has been an in
reased fo
us on the fabri
ation of new spintroni
devi
es
based on the tunnel magnetoresistan
e ee
t (TMR)1 and the re
ently dis
overed spin torque
ee
t (ST)2 in multilayered stru
tures
onsisting of several ferromagneti
nanolayers separated by thin insulating barriers. The geometri
parameters of su
h stru
tures also give us
the possibility to investigate some of their quasi-two-dimensional transport properties and
parti
ularly to
ompare the relationship between diagonal and o-diagonal (responsible for
EHE)
ondu
tivities in massive and above mentioned samples. This study is of great interest to the eld of spintroni
s sin
e quasi-two-dimensional EHE may provide an additional
me
hanism for re
ording and storing information in logi
devi
es. Fo
using on this aspe
t of
EHE we study both diagonal and o-diagonal (Hall)
ondu
tivities in a system
onsisting of
one ferromagneti
layer of thi
kness a pla
ed between two insulating layers and magnetized
in the dire
tion perpendi
ular to the interfa
es (zdire
tion).
The remainder of the paper is organized as follows. In Se
tion II EHE is attributed to the
me
hanism of skew-s
attering3 on the bulk and interfa
e impurities. We report our results
for the
ondu
tivity tensor in
luding size ee
t terms
al
ulated within the framework of the
Kubo formalism and
ompare the quasi-two-dimensional Hall resistan
e H
2D with that of a
massive sample H
bulk . Se
tion III dis
usses the nonideality of the interfa
es and the existen
e
of volume defe
ts that inuen
e the form of
urrent lines. We propose a new me
hanism
of EHE (we will refer to it as the geometri
me
hanism of EHE ) due to these defe
ts using
the diusion equation4 and taking into a
ount that the diusion
oe
ient has o-diagonal
omponent proportional to the spin-orbit intera
tion. We summarize our results and oer
some
on
lusions in Se
tion IV.
jx = xy Ey + xx ExH = 0
yx
H
2D,bulk =
2
yy xx + yx
(1)
(2)
where are diagonal and o-diagonal
ondu
tivities, ExH is the Hall eld. For the
al
ulation of H
2D,bulk we will use the Kubo formula with vertex
orre
tions responsible for the
transverse
omponent of the
urrent:
=
~e2 X
G+
(zz )G (z z)
a40
z
(3)
where ~ is the velo
ity ve
tor along the interfa
e, G+0 (zz ), G0 (zz ) are advan
ed and
retarded Green's fun
tions in mixed
oordinate-momentum representation. To
al
ulate the
y x
omponent of the
ondu
tivity tensor we will use the perturbation theory and will
take into a
ount only the
orre
tions in linear order of the spin-orbit intera
tion:
+
G+
(zz ) = G0 (zz ) + G0 (zz )
+
so
z ) G+
T
z ) + H
(~
(~
0 (z z )
so
z ) = iso (~z ) a20 mz [ ]z = iso (~
z ) a20 mz x y x y
H
(~
(4)
(5)
+
so
z) and H
z) are the s
attering matrix and the spin-orbit intera
tion,
orwhere T
(~
(~
respondently, dependant on the type of atom in (~z) position ; mz is the unit ve
tor along
the magnetization, so
m is the spin-orbit parameter and a0 is the latti
e
onstant. It follows
so
from Eq. (5) that H (~z ) = Hso (~z ).
For the T matrix in one-site approximation we
an write down:
T (~z) =
n (z)
1 (n (z)) G (~n z, ~n z)
n
X
z) =
ei( )(~~m ) so
so
m
(~
ei( )(~~n )
(6)
(7)
a20
2
a0
be found from the system of self-
onsistent equations. The rst equation of the system is
valid for s
attering on both bulk and interfa
e impurities:
cA
B (z)
A (z)
+ cB
=0
1 (A (z)) G0 (~n z, ~n z)
1 (B (z)) G0 (~n z, ~n z)
(8)
while the se
ond one is written in the form
orresponding to the interfa
e s
attring sin
e we
are interested in
al
ulation of the interfa
e
oherent potential:
G (~n z, ~n z) =
G0 (~n z, ~n z)
1 (z) G0 (~n z, ~n z)
(9)
For the
al
ulation of xx , yy we will use Eq. (3) with Green's fun
tions diagonal on
and renormalized on the
oherent potential. For o-diagonal
omponent averaging on the
impurities distribution gives:
yx =
~3 e2 Mz X 2 2 +
+
2
2 +
Im T
~n z )so
~n z )
G
(z
z
)
G
(zz
)
(
(
y x
2 2
a0 m
(10)
~n
where ~n z is the impurity position. We keep in Eq. (10) only the main term with n = m.
For the binary AB stru
ture and purely random distribution of A, B summing over ~n
will give . It is
onvenient to divide so into average and s
attering parts:
so
so
so
so
so
so
A = cA A + cB B + cB A cB B = + cB
cA so
so = cA so + cB so + cA so cA so =
B
(11)
(12)
cA
+ cB
1 (A (z)) G (~n z, ~n z)
1 (B (z)) G (~n z, ~n z)
B (z)
A (z)
so
+ cA cB
1 (A (z)) G (~n z, ~n z) 1 (B (z)) G (~n z, ~n z)
(13)
A
ording to Eq. (8) and Eq. (9) we only take the imaginary part of the last term in Eq.
(13). We rewrite Eq. (13) with renormalized Green's fun
tion:
(A (z)) (1 (z) G0 (~n z, ~n z))
1 X
so
so
hTn (z)n (z)i cA cB Im
Im
N n
1 A G0 (~n z, ~n z)
1 B G0 (~n z, ~n z)
G0 (~n z, ~n z) F0 (z)
(14)
(15)
(E, z) = +
= cA A + cB B ,
cA cB 2 F (E, z)
1 (
(E, z)) F (E, z)
(16)
= cA B + cB A ,
(17)
= A B
1
ImF
2
(1 cBbulk bulk ReF ) (1 + cAbulk bulk ReF )2
(18)
For the interfa
e values the full self-
onsistent s
heme is ne
essary. For both bulk and
interfa
e we suppose that the real part of the
oherent potential just represents the renormalization of ele
tron spe
trum so
an be
onsidered as purely imaginary.
The zero order Green's fun
tion found from S
hrdinger equation in z representation
is (we will further use the units with energy dimension [L] = A ):
G+
0 (0 < z < z < z1 ) =
1
2
(19)
k1 =
kF
2
2kF
+i
c1 + id1
l1
(20)
s
1
2
2
2
2
1
4k
c1 =
kF 2 + F +
kF 2
l1
2
s
1
2
2
2
2
1
4k
d1 =
kF 2 + F
kF 2
l1
2
q
2m
q = q02 + 2 ,
q02 = 2 (U EF )
~
(21)
(22)
(23)
where 0 and z1 are the oordinates of the left and right interfa es, a is the layer thi kness; kF ,
l1 are the Fermi momentum and the mean free path for spin "up", respe
tively, c1 d1 = l1F
(for spin "down" we will use index 2 ); U is the height of the potential barrier.
The poles of the Green's fun
tion in Eq. (19) dene the quantized energy spe
trum of
the thin ferromagneti
layer.
G0 (z0) G0 (0z )
1 G0 (00)
(24)
Integrating over z from 0 to z for z < z and from z to a for z > z gives the
ondu
tivity
in the units ohm1 cm1 :
Z 3
dNom
0 l1 108
xx =
(25)
c1 Den
2kF
q 2 + c21 + ||2 + 2qRe sinh 2d1 a + 2c1 |Im| cosh 2d1 a
+ 2c1 Im q 2 + c21 cosh 2d1 (z a) + 2 sinh2 d1 z (cos 2c1 (z a) + 2qc1 sin 2c1 (z a))
2c1 (q + Re) q 2 + c21 sinh 2d1 (z a) sin 2c1 z + q 2 + c21 + ||2 + 2qRe
q 2 + c21 sinh 2d1 (z a) cos 2c1 z sinh 2d1 z q 2 c21 cos 2c1 (z a) + 2qc1 sin 2c1 (z a)
Nom = q 2 + c21
(26)
Den = q 2 + c21
q 2 + c21 + ||2 + 2qRe cosh 2d1 a + 2c1 |Im| sinh 2d1 a
q 4 6q 2 c21 + c41 + ||2 + 2qRe q 2 c21 4qc21 Re cos 2c1 a
2qc1 2 q 2 c21 + qRe + ||2 sin 2c1 a
(27)
4x104
-1
-1
(ohm . cm )
5x104
xx
3x104
2x104
10
a (
15
20
Figure 1: Averaged diagonal
ondu
tivity as a fun
tion of a (thi
kness): < xx > (a) for kF =
, l2 = 60(A)
, c = 0.3 (see Eq. (28))
1.1(A 1 ), kF = 0.6(A 1 ), l1 = 100(A)
e
= 10
(ohm1 ) is the elementary
ondu
tivity of one
hannel.
where 0 = 2~
13.6
For large enough layer thi
kness we
an average Eq. (25) over os
illations so that the
averaged
ondu
tivity is:
3
0 l1 108
xx =
2kF
#
"
3 d
l1
|Im| c1 sinh 2d1 a
1
c1
a q 2 + c21 + ||2 + 2qRe sinh 2d1 a + 2c1 |Im| cosh 2d1 a
(28)
The rst term in Eq. (28) is the
ondu
tivity of the massive sample and the se
ond one
is due to the quasi-
lassi
al size ee
t. The full
ondu
tivity representing the sum of two
spin
hannels is shown on Fig. (1) as a fun
tion of the layer thi
kness.
B. Cal ulation of the o-diagonal ondu tivity due to the spin-orbit interfa e s attering
(z) using Eq. (10) with Green's fun
tion dened by Eq. (24)
Now we will
al
ulate xy
xy
=
Z
0 l1 a40 108
2 2 kF
3 d
ik1 a (q ic )2 1 +
(q + ic1 )2 1 + q+ic
e
e
1
1
qic1
2
ik1 a (q ic )2 1 +
e
(q + ic1 )2 1 + q+ic
e
1
qic1
1
15
xy
-1
-1
(ohm . cm )
20
10
5
5
10
a (
15
20
Figure 2: O-diagonal
ondu
tivity as a fun
tion of a (thi
kness): xy (a) for kF = 1.1(A 1 ),
, l2 = 60(A)
, c = 0.3, so = 0.05(A 1 ) (see Eq. (29))
kF = 0.6(A 1 ), l1 = 100(A)
This
ondu
tivity os
illates with the thi
kness and the distan
e from the interfa
e z = 0.
Its behavior be
omes more
lear after averaging over os
illations:
Z
0 l1 a40 108
Im hT (~n 0) so (~n 0)i sinh 2d1 a
3
dc
xy =
1
q 2 + c21 + | |2 + 2qRe sinh 2d1 a + 2c1 Im cosh 2d1 a
8 2 kF
Z
cosh 2d1 (z a)
3 d
2
2
q 2 + c1 + | | + 2qRe sinh 2d1 a + 2c1 Im cosh 2d1 a
(30)
The same is done for spin "down". The sum of these two terms is shown on Fig. (2).
de
reases with z a sin
e the fun
tions cosh 2d1 (za) have maximum
It is
lear that xy
over these fun
tions gives the fa
tor la1 so for innite a this
values at z = 0. Averaging xy
term tends to zero.
+ xy
(see Fig. (3)) using Eq. (10) with
We also
al
ulate the bulk
ondu
tivity xy
additional integration over z and bulk s
attering parameters with the bulk
oherent poten2
tial in Bohrn approximation bulk = icbulk (1 cbulk )bulk
ImF bulk (zz). In the absen
e of the
interfa
ial s
attering this approa
h gives us:
200
xy
bulk
-1
-1
(ohm . cm )
300
100
10
a (
15
20
bulk
xy
8Z
Z 3
2
0 l12 a30 Im T bulk so
3 d (q 2 + c21 ) sinh 2d1 a
d 1 n 2
bulk 10
2 2
=
q
+
c
1
2
c1
Den
c1 Den
8 2 kF
sinh 2d1 a q 4 c41 (sinh 2d1 z cos 2c1 (z a) sinh 2d1 (z a) cos 2c1 z)
+2qc1 (sinh 2d1 z sin 2c1 (z a) + sinh 2d1 (z a) sin 2c1 z)}
(31)
2
q 4 6q 2 c21 + c41 cos 2c1 a + 4c1 q q 2 c21 sin 2c1 a
(32)
8 Z
2
0 l12 a30 Im T bulk so
3 d
bulk 10
=
c1
8 2 kF2
(33)
This
ondu
tivity has an os
illating behavior for the thin layer but tends to the
onstant
value when a whi
h
oin
ides with its value for the massive sample. If we take into
bulk
a
ount the interfa
ial s
attering the expression for xy
be
omes too
ompli
ated so we
H
xy
bulk
al
ulated using
don't show it here. But the thi
kness dependen
es of xy and = xx
the full formula with renormalized Green's fun
tion are presented at Fig. (4) and Fig. (5),
1 bulk = 0.01, bulk = 1(A 1 ).
orrespondently. The bulk parameters are: so
bulk = 0.03(A ), c
250
xy
bulk
-1
-1
(ohm . cm )
300
200
150
10
15
a (
20
Figure 4: Bulk o-diagonal
ondu
tivity with interfa
ial s
attering as a fun
tion of a (thi
kness):
bulk (A) for k = 1.1(A 1 ), k = 0.6(A 1 ), l = 100(A)
, l2 = 60(A)
xy
1
F
F
-2
-2
1.0x10
xy
xx
1.5x10
-3
5.0x10
10
a (
15
20
1
Figure 5: Hall angle = xx as a fun
tion of a (thi
kness); bulk parameters: so
bulk = 0.03(A ),
cbulk = 0.01, bulk = 1(A 1 ); interfa
e parameters: so = 0.05(A 1 ), c = 0.3, = 1.5(A 1 )
H
xy
defe
ts whi
h will be modeled as
ylinders of radius R so that the
urrent lines in the vi
inity
of these defe
ts follow their shape.
Diusion equations for
harge and spin
urrents in the absen
e of pre
ession are:
n jex jey
+
+
=0
t
x
y
m
~
j x
j y
m
~
+ m + m =
t
x
y
sf
n
t
m
~
t
(34)
(35)
n
m
m
n
Dxx
Dxy
Dxy
x
x
y
y
n
m
n
m
jey = yy 0 + yx E Dyy
Dyy
Dyx
Dyx
y
y
x
x
m
m
n
n
x
Dxx
Dxy
Dxy
jm
= xx E Dxx
x
x
y
y
n
m
n
m
y
jm
= yy 0 + yx E Dyy
Dyy
Dyx
Dyx
y
y
x
x
jex = xx E Dxx
(36)
(37)
(38)
(39)
~ = {E, 0, 0}, m
Here we take into a
ount that E
~ = {0, 0, m} are the ele
tri
eld and
spin a
umulation
orrespondently, D are the
omponents of diusion
oe
ient tensors.
O-diagonal
omponents Dxy and Dyx of these tensors are proportional to the spin-orbit
intera
tion and they are antisymmetri
al in the x y transposition. For a metal with the
ubi
symmetry xx = yy , Dxx = Dyy D0 . Then we insert Eq. (36)-(39) into Eq. (34)
and Eq. (35) and after some manipulations we obtain two equations:
n = m
m
n + m =
sf
m
=0
2sf
(40)
(41)
(42)
For the
ylindri
al defe
t shape it is
onvenient to sear
h for solution in polar
oordinates
so we
an rewrite Eq. (42):
1
r r
m
r
r
1 2m
m
1 2m
m
2 m 1 m
+ 2
2
+
+ 2
2 =0
2
2
2
r
sf
r
r r
r
sf
(43)
where is the angle between xaxe and the radius-ve
tor ~r with the
oordinates (x, y).
The solution of Eq. (43) is:
m = m1 (r) m2 ()
m2 () = A1n cos n + A2n sin n
10
(44)
(45)
As
2 m2
2
+ 2 m1 = 0
m2 ()
r 2
r r
2sf
r
(46)
r
sf
(47)
r
sf
(48)
n = m + n0
n0 = 0
1
rn
(51)
Taking into a
ount Eq. (40) we
an rewrite Eq. (36) and Eq. (37):
n0
n0
Dxy
x
y
n0
n0
+ Dyx
jey = yx E Dyy
y
x
jex = xx E Dxx
(52)
(53)
Now it is
onvenient to use the polar
oordinate system and to write down r and
proje
tions of the
urrents. Then we
an use the boundary
onditions to nd unknown
oe
ients. These proje
tion are:
0
jre
= xx E cos + xy E sin
(54)
(usual term)
jre = Dxx
n0
n0
n0
n0
cos Dxy
cos Dyy
sin + Dxy
sin
x
y
y
x
(55)
11
(56)
(57)
Using the expressions for derivatives of r, over x, y , whi
h is not too di
ult to obtain,
we write down the
harge and spin
urrents in polar
oordinates:
n r n
n
n r
+ sin
+
+
jre = D0 cos
r x x
r y y
n r
n r n
n
Dxy cos
sin
+
+
r x x
r y y
n
n
Dxy
= D0
r
r
n
n
Dxy
r
r
m
m
Dxy
= D0
r
r
(58)
n
jrm
= D0
(59)
m
jrm
(60)
0
jrm
= xx E cos + yx E sin
(61)
To nd the unknown
oe
ients in Eq. (48) and Eq. (51) we will use the boundary
onditions on the surfa
e of the
ylinder representing that rproje
tion of
urrents are
equal to zero:
X
n0
n
n0
|r=R + Dxy
|r=R = D0
(C1n cos n + C2n sin n) n+1
r
R
R
n
X
n
Dxy
(C1n sin n C2n cos n) n+1
R
n
n
jR0
+ jRn = 0 D0
(62)
(63)
(64)
with solution
C11 =
n0 =
D0 xy + Dxy xx
D0 xx Dxy xy
, C21 =
2
2
2
D0 + Dxy
D02 + Dxy
(65)
(66)
(67)
12
I1 (x)
2
= lim
(I1 I+1 ) = lim
I (x) =
(69)
0 2 sin ( + 1) x
0 sin x x
x
x
K1 (x) = lim
where x rsf , x
= 1sf .
r
Inserting Eq. (68)-(69) in Eq. (67) we get:
I1
R
I0 sf
+ Dxy (A11 sin A21 cos )
R2
(70)
Exx = D0 A11
(71)
Exy
(72)
r
r
ER xx D0 I1 sf R + xy Dxy I0 sf sf
=
2
2
D0 I1 rsf R + Dxy I0 rsf sf
r
2
ER xx Dxy I0 sf sf xy D0 I1 rsf R
=
2
2
D0 I1 rsf R + Dxy I0 rsf sf
2
A11
A21
ER2 sf I0 rsf
m =
2
2
r
r
r
D0 I1 sf R + Dxy I0 sf sf
r
r
R + xy Dxy I0
sf
cos xx D0 I1
sf
sf
r
r
sf xy D0 I1
R
+ sin xx Dxy I0
sf
sf
(73)
(74)
(75)
Now we
an dene the additional Hall eld due to this
ylindri
al interfa
e defe
t
onsidering that Hall ele
trodes are the surfa
es with
oordinates y = a and y = a. This eld
is proportional to n(a) n(a), n = m + n0 , r = |sina | . After integrating over from 0
to for the left surfa
e and from to 2 for the right one we will have:
ER2
n0 (a) n0 (a) = 2
a
ER2 (Dxy xx + D0 xy )
sin2 (Dxy xx + D0 xy )
=
(76)
2
2
D02 + Dxy
a D02 + Dxy
13
nm (a) nm (a) =
2 ER
a
sin2 xx Dxy I0 rsf sf xy D0 I1 rsf R
(77)
d
2
2
r
r
D0 I1 sf R + Dxy I0 sf sf
At last, we have to multiply Eq. (76) and Eq . (77) by the
on
entrations of defe
ts and
ele
tron
harge.
IV. CONCLUSION
It was shown that due to the additional s
attering of ele
trons on the defe
ts of the
metal-insulator interfa
es the total
ondu
tan
e de
reases. From Eq. (28) it follows that
for small values of the ratio al the bulk
ondu
tivity is
ompletely suppressed and ee
tive
ondu
tivity is proportional to the ee
tive s
attering length on the interfa
es instead of the
bulk mean free path. Hall
ondu
tivity, if we don't take into a
ount the additional s
ews
attering on the interfa
e, de
reases with de
reasing the thi
kness of the ferromagneti
metalli
layer. However the
ontribution to the Hall
ondu
tivity due to the additional
s
ew-s
attering on the interfa
e in
reases. So the important
hara
teristi
of the
onsidered
xy
xy
devi
e, Hall angle xx
= xx
, is larger for the thin ferromagneti
layer
ompared to the bulk
layer. Besides that, the inuen
e of insulator
olumns penetrating into the metalli
layer
may further in
rease the value of the Hall ee
t.
A
knowledgments
N. Ryzhanova and A. Vedyayev are grateful to SPINTEC for hospitality. This work was
partially supported by the Russian Foundation for Basi
Resear
h.
1
2
3
4
5
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